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Author |
Post, V.E.A.; Vassolo, S.I.; Tiberghien, C.; Baranyikwa, D.; Miburo, D. |
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Title |
Weathering and evaporation controls on dissolved uranium concentrations in groundwater – A case study from northern Burundi |
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Journal Article |
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Year |
2017 |
Publication |
Science of The Total Environment |
Abbreviated Journal |
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Volume |
607-608 |
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281-293 |
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Keywords |
Geochemical modelling, Hydrochemistry, Lake Tshohoha South, Public health, Radionuclides, Water supply |
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Abstract |
The potential use of groundwater for potable water supply can be severely compromised by natural contaminants such as uranium. The environmental mobility of uranium depends on a suite of factors including aquifer lithology, redox conditions, complexing agents, and hydrological processes. Uranium concentrations of up to 734μg/L are found in groundwater in northern Burundi, and the objective of the present study was to identify the causes for these elevated concentrations. Based on a comprehensive data set of groundwater chemistry, geology, and hydrological measurements, it was found that the highest dissolved uranium concentrations in groundwater occur near the shores of Lake Tshohoha South and other smaller lakes nearby. A model is proposed in which weathering and evapotranspiration during groundwater recharge, flow and discharge exert the dominant controls on the groundwater chemical composition. Results of PHREEQC simulations quantitatively confirm this conceptual model and show that uranium mobilization followed by evapo-concentration is the most likely explanation for the high dissolved uranium concentrations observed. The uranium source is the granitic sand, which was found to have a mean elemental uranium content of 14ppm, but the exact mobilization process could not be established. Uranium concentrations may further be controlled by adsorption, especially where calcium-uranyl‑carbonate complexes are present. Water and uranium mass balance calculations for Lake Tshohoha South are consistent with the inferred fluxes and show that high‑uranium groundwater represents only a minor fraction of the overall water input to the lake. These findings highlight that the evaporation effects that cause radionuclide concentrations to rise to harmful levels in groundwater discharge areas are not only confined to arid regions, and that this should be considered when selecting suitable locations for water supply wells. |
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0048-9697 |
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THL @ christoph.kuells @ post_weathering_2017 |
Serial |
132 |
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Author |
Vogel, J.C.; Talma, A.S.; Heaton, T.H.E.; Kronfeld, J. |
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Title |
Evaluating the rate of migration of an uranium deposition front within the Uitenhage Aquifer |
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Journal Article |
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Year |
1999 |
Publication |
Journal of Geochemical Exploration |
Abbreviated Journal |
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Volume |
66 |
Issue |
1 |
Pages |
269-276 |
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Keywords |
redox changes in aquifer, sandstone-type uranium deposit, South Africa, uranium series |
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Abstract |
The solubility of uranium in groundwater is very sensitive to changes in redox conditions. Many secondary (sandstone-type) uranium deposits have been formed when soluble U has precipitated after encountering reducing conditions in the subsurface. In the groundwater of the Uitenhage Aquifer (Cape Province, South Africa), 238U-series isotopes were used to assist in studying the history of the reducing barrier. Uranium isotopes were used to determine the present position of the barrier. Radium and radon were used to evaluate the path of migration that the front of the oxygen depletion zone has taken over the past 105 years. During this time the reducing barrier has moved, leaving in its wake a trail of U in various stages of secular equilibrium with its daughter 230Th. The 226Ra daughter of 230Th is not very mobile. Its growth upon the aquifer wall is reflected in the Rn content of the water. This in turn, due to the relatively great age of the water, indicates the extent of the 230Th ingrowth (from precipitated U) that took place before the barrier migrated. |
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0375-6742 |
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THL @ christoph.kuells @ vogel_evaluating_1999 |
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126 |
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Author |
Lightfoot, D.R. |
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Title |
Moroccan khettara: Traditional irrigation and progressive desiccation |
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Journal Article |
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Year |
1996 |
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Geoforum |
Abbreviated Journal |
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27 |
Issue |
2 |
Pages |
261-273 |
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A 300 km network of khettara (qanat) subsurface irrigation channels was excavated in the Tafilalt basin beginning in the late 14th century. More than 75 of these chains provided perennial water following the breakup of the ancient city of Sijilmassa. Khettara continued to function for much of the northern oasis until the early 1970s, when new technologies and government policies forced changes. Data on origins, maintenance, and current use were collected from archival sources, aerial photographs, Landsat imagery, and from interviews. Insufficient water resources and unsustainable practices have dramatically lowered the water table, drying up khettara. This has resulted in a loss of local control over water resources, abandonment of a sustainable irrigation system, and progressive desiccation. |
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0016-7185 |
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THL @ christoph.kuells @ Lightfoot1996261 |
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257 |
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Author |
Heaton, T.H.E. |
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Title |
Sources of the nitrate in phreatic groundwater in the western Kalahari |
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Journal Article |
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Year |
1984 |
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Journal of Hydrology |
Abbreviated Journal |
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67 |
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1 |
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249-259 |
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Elevated levels of nitrate occur in phreatic groundwater in the western Kalahari, Namibia. Nitrate in water containing 0.4–3.1 meq NO−3l−1, of widespread occurrence, has δ15N values in the range +4.9 to +8.0‰, suggesting natural derivation from the soil. The sporadic occurrence of very high levels of nitrate (> 4 meq NO−3l−1), which has δ15N between +9.3 to +18.7‰, reflects pollution derived from animal waste. The importance of considering the possible isotopic effects of denitrification, and the significance of leaching in the nitrogen budget of the Kalahari soil, are also discussed. |
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0022-1694 |
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THL @ christoph.kuells @ Heaton1984249 |
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278 |
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Author |
Heaton, T.H.E.; Talma, A.S.; Vogel, J.C. |
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Title |
Origin and history of nitrate in confined groundwater in the western Kalahari |
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Journal Article |
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Year |
1983 |
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Journal of Hydrology |
Abbreviated Journal |
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62 |
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1 |
Pages |
243-262 |
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Data are presented for nitrate, dinitrogen and argon concentrations and 15N14N ratios in groundwater, with radiocarbon ages up to 40,000 yr. for three confined sandstone aquifers in the western Kalahari of South West Africa/Namibia. The nitrate is probably generated within the soil of the recharge areas, and its production rate during the period 3000-40,000 B.P. has remained between 0.5 and 1.6 meq NO−3l−1 of recharge water, with ° 15N between + 4 and + 8‰. Variations in the amount of nitrate and of “excess air” in groundwater recharge are found, and can only reflect changes in the environmental conditions during recharge. They must therefore be caused by the climatic changes that have taken place during the past 25,000 yr. |
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0022-1694 |
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THL @ christoph.kuells @ heaton_origin_1983 |
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95 |
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Author |
Heaton, T.H.E.; Talma, A.S.; Vogel, J.C. |
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Title |
Origin and history of nitrate in confined groundwater in the western Kalahari |
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Journal Article |
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1983 |
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Journal of Hydrology |
Abbreviated Journal |
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62 |
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1 |
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243-262 |
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Abstract |
Data are presented for nitrate, dinitrogen and argon concentrations and 15N14N ratios in groundwater, with radiocarbon ages up to 40,000 yr. for three confined sandstone aquifers in the western Kalahari of South West Africa/Namibia. The nitrate is probably generated within the soil of the recharge areas, and its production rate during the period 3000-40,000 B.P. has remained between 0.5 and 1.6 meq NO−3l−1 of recharge water, with ° 15N between + 4 and + 8‰. Variations in the amount of nitrate and of “excess air” in groundwater recharge are found, and can only reflect changes in the environmental conditions during recharge. They must therefore be caused by the climatic changes that have taken place during the past 25,000 yr. |
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0022-1694 |
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THL @ christoph.kuells @ Heaton1983243 |
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282 |
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Author |
Uhrie, J.L.; Drever, J.I.; Colberg, P.J.S.; Nesbitt, C.C. |
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Title |
In situ immobilization of heavy metals associated with uranium leach mines by bacterial sulfate reduction |
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Journal Article |
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1996 |
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Hydrometallurgy |
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43 |
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1 |
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231-239 |
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Laboratory experiments with mixed populations of sulfate-reducing bactreria were shown to mediate the removal of milligrams/liter concentrations of uranium, selenium, arsenic and vanadium from aqueous solution via reduction, precipitation and adsorption. Results of laboratory experiments with active sulfidogenic biomass suggest that injection of sulfate and a source of carbon could enhance anaerobic microbial activity in and around uranium leach mines leading to in situ immobilization contaminating metals. |
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0304-386x |
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THL @ christoph.kuells @ uhrie_situ_1996 |
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197 |
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Author |
Rubin, R. |
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Title |
Water conservation methods in Israel’s Negev desert in late antiquity |
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Journal Article |
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Year |
1988 |
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Journal of Historical Geography |
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14 |
Issue |
3 |
Pages |
229-244 |
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Settlement in Israel’s Negev desert historically has been dependent on water conservation techniques. Fieldwork carried out on settlement sites constructed during the Byzantine period, when agriculture and trade flourished, revealed a variety of water installations some of which are in use today. Perennial springs in the Negev are generally small and difficult of access. Cisterns were the most common conservation devices and came in both large, enclosed and single, open forms. Cisterns were common particularly in the towns, where they were usually built as part of house foundations. Dams were discovered at several sites but proved to be inefficient and easily abandoned because of evaporation and siltation problems. Public reservoirs were part of the structure of the largest towns and were open and among the larges structures uncovered at settlement sites. Wells were distributed widely throughout the desert and were part of the only conservation system that did not depend directly on surface rainfall. A qanat system was located in the eastern Negev dating from the late settlement period before the area was abandoned at the turn of the eighth century. These various water systems raise questions about their builders and their origins, and suggests that builders originating in more humid Mediterranean environments tended to produce less adaptable installations than builders derived from the south or the east. |
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0305-7488 |
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THL @ christoph.kuells @ Rubin1988229 |
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262 |
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Author |
Kharaka, Y.; Harmon, R.; Darling, G. |
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Title |
W. Mike Edmunds (1941–2015) |
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Journal Article |
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Year |
2015 |
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Applied Geochemistry |
Abbreviated Journal |
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59 |
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225-226 |
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0883-2927 |
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THL @ christoph.kuells @ kharaka_w_2015 |
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103 |
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Author |
Hdeib, R.; Aouad, M. |
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Title |
Rainwater harvesting systems: An urban flood risk mitigation measure in arid areas |
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Journal Article |
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Year |
2023 |
Publication |
Water Science and Engineering |
Abbreviated Journal |
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16 |
Issue |
3 |
Pages |
219-225 |
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Keywords |
Rainwater harvesting, Urban floods, Flood map, Hydrodynamic model, Built environment, Arid areas |
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Abstract |
Rainwater harvesting (RWH) systems have been developed to compensate for shortage in the water supply worldwide. Such systems are not very common in arid areas, particularly in the Gulf Region, due to the scarcity of rainfall and their reduced efficiency in covering water demand and reducing water consumption rates. In spite of this, RWH systems have the potential to reduce urban flood risks, particularly in densely populated areas. This study aimed to assess the potential use of RWH systems as urban flood mitigation measures in arid areas. Their utility in the retention of stormwater runoff and the reduction of water depth and extent were evaluated. The study was conducted in a residential area in Bahrain that experienced waterlogging after heavy rainfall events. The water demand patterns of housing units were analyzed, and the daily water balance for RWH tanks was evaluated. The effect of the implementation of RWH systems on the flood volume was evaluated with a two-dimensional hydrodynamic model. Flood simulations were conducted in several rainfall scenarios with different probabilities of occurrence. The results showed significant reductions in the flood depth and flood extent, but these effects were highly dependent on the rainfall intensity of the event. RWH systems are effective flood mitigation measures, particularly in urban arid regions short of proper stormwater control infrastructure, and they enhance the resilience of the built environment to urban floods. |
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1674-2370 |
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THL @ christoph.kuells @ Hdeib2023219 |
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242 |
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