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Author (down) Zhou, Y.; Li, G.; Xu, L.; Liu, J.; Sun, Z.; Shi, W. url  openurl
  Title Uranium recovery from sandstone-type uranium deposit by acid in-situ leaching – an example from the Kujieertai Type Journal Article
  Year 2020 Publication Hydrometallurgy Abbreviated Journal  
  Volume 191 Issue Pages 105209  
  Keywords Acid in-situ leaching, Sandstone-type uranium deposit, Uranium deportment in the ore, Uranium recovery, Water-rock interaction  
  Abstract The factors influencing uranium recovery in water-rock systems during acid in-situ leaching (ISL) were studied at the Kujieertai uranium deposit in Xinjiang. Using an ISL unit, a field leach trial (FLT) had been carried out to test the sequential effects of a leaching solution without oxidant (H2SO4 solution 4–8 g/L) and a leaching solution with oxidant (H2SO4 3–7 g/L, and Fe (III) 2–6 g/L). The observation of the leaching process revealed clearly defined stages of uranium release from the solid mineral to solution. Uranium mobilization from solid mineral into solution can be described in four stages. At the beginning of the acid ISL process, there was no oxidant to be added to the leaching solution and the desorption of hexavalent uranyl ions in the open pores, as well as dissolution of hexavalent uranium minerals, led to a short-term peak in the pregnant solution, which happened while pH decreased from about 5.3 to 2.62. Following the depletion of the adsorbed hexavalent uranium and a decline in uranium dissolution intensity, the addition of Fe(III) facilitated the oxidation of tetravalent uranium, which enabled intensive uranium mobilization again. During this process, the dissolution of uranium had a strong positive correlation with the reduction of Fe(III) and Eh in the leach solution. Beside hydrochemical factors, the deportment of uranium was also an important factor affecting uranium recovery. Uranium located in the open pores can be completely exposed to the solution and the mobilization intensity was significantly affected by hydrogeochemical conditions; but the uranium present in microfissures and in the ore matrix could not be fully exposed to the solution, so, their dissolution intensity was primarily controlled by corrosion and permeability of the ore. In general, the hydrogeochemical conditions and the deportment of uranium were the external and internal factors that significantly affected the dissolution and recovery of uranium in the early and middle stages of the FLT. However, in the latest stages, due to uranium depletion, enhancing the chemical potential of the leaching solution, specifically acidity and/or the amount of oxidant, had little improvement on uranium recovery.  
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  Series Volume Series Issue Edition  
  ISSN 0304-386x ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ zhou_uranium_2020 Serial 205  
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Author (down) Zhao, Y.; Li, X.; Lei, L.; Chen, L.; Luo, Z. url  openurl
  Title Permeability evolution mechanism and the optimum permeability determination of uranium leaching from low-permeability sandstone treated with low-frequency vibration Type Journal Article
  Year 2023 Publication Journal of Rock Mechanics and Geotechnical Engineering Abbreviated Journal  
  Volume 15 Issue 10 Pages 2597-2610  
  Keywords Chemical reactive rate, Low-frequency vibration, Low-permeability sandstone, Optimum permeability, Permeability evolution mechanism, Uranium migration  
  Abstract Low-frequency vibrations can effectively improve natural sandstone permeability, and higher vibration frequency is associated with larger permeability. However, the optimum permeability and permeability evolution mechanism for uranium leaching and the relationship between permeability and the change of chemical reactive rate affecting uranium leaching have not been determined. To solve the above problems, in this study, identical homogeneous sandstone samples were selected to simulate low-permeability sandstone; a permeability evolution model considering the combined action of vibration stress, pore water pressure, water flow impact force, and chemical erosion was established; and vibration leaching experiments were performed to test the model accuracy. Both the permeability and chemical reactions were found to simultaneously restrict U6+ leaching, and the vibration treatment increased the permeability, causing the U6+ leaching reaction to no longer be diffusion-constrained but to be primarily controlled by the reaction rate. Changes of the model calculation parameters were further analyzed to determine the permeability evolution mechanism under the influence of vibration and chemical erosion, to prove the correctness of the mechanism according to the experimental results, and to develop a new method for determining the optimum permeability in uranium leaching. The uranium leaching was found to primarily follow a process consisting of (1) a permeability control stage, (2) achieving the optimum permeability, (3) a chemical reactive rate control stage, and (4) a channel flow stage. The resolution of these problems is of great significance for facilitating the application and promotion of low-frequency vibration in the CO2 + O2 leaching process.  
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  Series Editor Series Title Abbreviated Series Title  
  Series Volume Series Issue Edition  
  ISSN 1674-7755 ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ zhao_permeability_2023 Serial 198  
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Author (down) Zhang, Y.; Liu, X.; Yuan, S.; Song, J.; Chen, W.; Dias, D. url  openurl
  Title A two-dimensional experimental study of active progressive failure of deeply buried Qanat tunnels in sandy ground Type Journal Article
  Year 2023 Publication Soils and Foundations Abbreviated Journal  
  Volume 63 Issue 3 Pages 101323  
  Keywords Qanat tunnel, Sand, Failure effect, Soil arching, Model test  
  Abstract As an ancient underground hydraulic engineering facility, the Qanat system has been used to draw groundwater from arid regions. A qanat is a horizontal tunnel with a slight incline that draws groundwater from a higher location and delivers it to lower agricultural land. During long-term water delivery, the qanat tunnel has experienced different degrees of aging and collapse, which may result in the significant ground settlement and even disasters. This paper developed a two-dimensional laboratory system to investigate the influence of progressive failure on the stability of deeply buried qanat tunnels. The developed system is fully instrumented with a particle image velocimetry (PIV) system and earth pressure and displacement monitoring. A special cylindrical membrane tube is designed and connected to an advanced pressure–volume controller to simulate the step-wise failure process of the tunnel. Three model tests were conducted on a dry sand considering the buried qanat tunnels at three different depths. Experimental results clearly show the progressive evolution of soil arching effect in the dry sand associated with the progressive failure of the tunnels. The failure of the Qanat ground starts from the vault and develops upwards, which is closely related to the evolution of stress contour at three consecutive stages. Ground surface settlement and volume loss corresponding to three burial depths were compared. A deeply buried qanat tunnel has a small effect on surface settlement. Earth pressure evolution on the 2D plane shows the load redistribution when the qanat collapses. The maximum arch and the initial point of the limit state correspond to a volume loss of 12.5 % and 50 %, respectively. For the collapse of the deep buried qanat tunnel, ground earth pressure evolution can be divided into a stress-increasing region, stress-decreasing region, and no redistribution region. Furthermore, a multi trap-door model considering soil expansion is proposed to describe the progressive failure behavior and its effects.  
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  Series Volume Series Issue Edition  
  ISSN 0038-0806 ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ Zhang2023101323 Serial 274  
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Author (down) Zhang, H.; Gao, J.; Xu, L.; Zhang, X. url  openurl
  Title Case studies of radioactivity of drilling mud for in situ leaching uranium mining in China Type Journal Article
  Year 2022 Publication Journal of Environmental Radioactivity Abbreviated Journal  
  Volume 251-252 Issue Pages 106982  
  Keywords Drilling mud, Exemption management, In situ leaching, Radioactivity  
  Abstract The drilling mud from in situ leaching uranium mining is a type of low-radioactivity waste that contains natural nuclides and other harmful substances. In order to determine whether the drilling mud can meet the requirements of radioactive exemption management standards, field investigations and data simulations were conducted in this study. Two typical uranium mines were selected for onsite investigations. Drilling mud from different layers (i.e., the upper covering layer and ore-bearing layer) and from different stages (e.g., logging stage mud, drilling expansion stage mud, and mixed mud) was sampled. For each sample, the 238U and 226Ra concentrations of the solid components and the U and 226Ra concentrations of the supernatant were analyzed. The results revealed that the highest 238U and 226Ra concentrations of the solid components were 4122 Bq/kg and 4077 Bq/kg, while the 238U and 226Ra concentrations of the mixed drilling mud were all less than 300 Bq/kg. A radioactivity estimation model was established for scenario analysis. Exemption management screening lines of waste drilling mud, which can be used to classify and treat the drilling project according to the deposit’s grade and conditions, were proposed for in situ leaching drilling projects.  
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  Corporate Author Thesis  
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  Series Editor Series Title Abbreviated Series Title  
  Series Volume Series Issue Edition  
  ISSN 0265-931x ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ zhang_case_2022 Serial 191  
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Author (down) Zeng, S.; Song, J.; Sun, B.; Wang, F.; Ye, W.; Shen, Y.; Li, H. url  openurl
  Title Seepage characteristics of the leaching solution during in situ leaching of uranium Type Journal Article
  Year 2023 Publication Nuclear Engineering and Technology Abbreviated Journal  
  Volume 55 Issue 2 Pages 566-574  
  Keywords In situ leaching, Leaching solution viscosity, Seepage characteristics, Seepage pressure, Uranium-bearing sandstone  
  Abstract Investigating the seepage characteristics of the leaching solution in the ore-bearing layer during the in situ leaching process can be useful for designing the process parameters for the uranium mining well. We prepared leaching solutions of four different viscosities and conducted experiments using a self-developed multifunctional uranium ore seepage test device. The effects of different viscosities of leaching solutions on the seepage characteristics of uranium-bearing sandstones were examined using seepage mechanics, physicochemical seepage theory, and dissolution erosion mechanism. Results indicated that while the seepage characteristics of various viscosities of leaching solutions were the same in rock samples with similar internal pore architectures, there were regular differences between the saturated and the unsaturated stages. In addition, the time required for the specimen to reach saturation varied with the viscosity of the leaching solution. The higher the viscosity of the solution, the slower the seepage flow from the unsaturated stage to the saturated stage. Furthermore, during the saturation stage, the seepage pressure of a leaching solution with a high viscosity was greater than that of a leaching solution with a low viscosity. However, the permeability coefficient of the high viscosity leaching solution was less than that of a low viscosity leaching solution.  
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  Series Editor Series Title Abbreviated Series Title  
  Series Volume Series Issue Edition  
  ISSN 1738-5733 ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ zeng_seepage_2023 Serial 211  
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Author (down) Zeng, S.; Shen, Y.; Sun, B.; Zhang, N.; Zhang, S.; Feng, S. url  openurl
  Title Pore structure evolution characteristics of sandstone uranium ore during acid leaching Type Journal Article
  Year 2021 Publication Nuclear Engineering and Technology Abbreviated Journal  
  Volume 53 Issue 12 Pages 4033-4041  
  Keywords Acid method, In situ leaching, Nuclear magnetic resonance, Pore characteristic, Sandstone uranium ore  
  Abstract To better understand the permeability of uranium sandstone, improve the leaching rate of uranium, and explore the change law of pore structure characteristics and blocking mechanism during leaching, we systematically analyzed the microstructure of acid-leaching uranium sandstone. We investigated the variable rules of pore structure characteristics based on nuclear magnetic resonance (NMR). The results showed the following: (1) The uranium concentration change followed the exponential law during uranium deposits acid leaching. After 24 h, the uranium leaching rate reached 50%. The uranium leaching slowed gradually over the next 4 days. (2) Combined with the regularity of porosity variation, Stages I and II included chemical plugging controlled by surface reaction. Stage I was the major completion phase of uranium displacement with saturation precipitation of calcium sulfate. Stage II mainly precipitated iron (III) oxide-hydroxide and aluminum hydroxide. Stage III involved physical clogging controlled by diffusion. (3) In the three stages of leaching, the permeability of the leaching solution changed with the pore structure, which first decreased, then increased, and then decreased.  
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  Series Volume Series Issue Edition  
  ISSN 1738-5733 ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ zeng_pore_2021 Serial 199  
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Author (down) Zeng, S.; Shen, Y.; Sun, B.; Tan, K.; Zhang, S.; Ye, W. url  openurl
  Title Fractal kinetic characteristics of uranium leaching from low permeability uranium-bearing sandstone Type Journal Article
  Year 2022 Publication Nuclear Engineering and Technology Abbreviated Journal  
  Volume 54 Issue 4 Pages 1175-1184  
  Keywords Fractal characteristics, In-situ leaching, Leaching kinetics, Pore structure, Uranium mine  
  Abstract The pore structure of uranium-bearing sandstone is one of the critical factors that affect the uranium leaching performance. In this article, uranium-bearing sandstone from the Yili Basin, Xinjiang, China, was taken as the research object. The fractal characteristics of the pore structure of the uranium-bearing sandstone were studied using mercury intrusion experiments and fractal theory, and the fractal dimension of the uranium-bearing sandstone was calculated. In addition, the effect of the fractal characteristics of the pore structure of the uranium-bearing sandstone on the uranium leaching kinetics was studied. Then, the kinetics was analyzed using a shrinking nuclear model, and it was determined that the rate of uranium leaching is mainly controlled by the diffusion reaction, and the dissolution rate constant (K) is linearly related to the pore specific surface fractal dimension (DS) and the pore volume fractal dimension (DV). Eventually, fractal kinetic models for predicting the in-situ leaching kinetics were established using the unreacted shrinking core model, and the linear relationship between the fractal dimension of the sample’s pore structure and the dissolution rate during the leaching was fitted.  
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  Series Editor Series Title Abbreviated Series Title  
  Series Volume Series Issue Edition  
  ISSN 1738-5733 ISBN Medium  
  Area Expedition Conference  
  Notes Approved no  
  Call Number THL @ christoph.kuells @ zeng_fractal_2022 Serial 193  
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Author (down) Zagana, E.; Obeidat, M.; Külls, C.; Udluft, P. url  doi
openurl 
  Title Chloride, hydrochemical and isotope methods of groundwater recharge estimation in eastern Mediterranean areas: a case study in Jordan Type Journal Article
  Year 2007 Publication Hydrological Processes: An International Journal Abbreviated Journal  
  Volume 21 Issue 16 Pages 2112-2123  
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  Publisher John Wiley & Sons, Ltd. Chichester, UK Place of Publication Editor  
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  Notes Approved no  
  Call Number THL @ christoph.kuells @ Zagana2007chloride Serial 29  
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Author (down) Zagana, E.; Külls, C.; Udluft, P.; Constantinou, C. url  doi
openurl 
  Title Methods of groundwater recharge estimation in eastern Mediterranean water balance model application in Greece, Cyprus and Jordan Type Journal Article
  Year 2007 Publication Hydrological Processes: An International Journal Abbreviated Journal  
  Volume 21 Issue 18 Pages 2405-2414  
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  Publisher John Wiley & Sons, Ltd. Chichester, UK Place of Publication Editor  
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  Notes Approved no  
  Call Number THL @ christoph.kuells @ Zagana2007methods Serial 30  
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Author (down) Zagana, E.; Külls, C.; Udluft, P. openurl 
  Title Der Wasserhaushalt des Aliakmonas Type Journal Article
  Year 2000 Publication Vom Wasser Abbreviated Journal  
  Volume 94 Issue Pages 29-39  
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  Notes Approved no  
  Call Number THL @ christoph.kuells @ Zagana2000saa Serial 34  
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