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Author |
Puri, S. |
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Title |
Chapter 9 – Transboundary aquifers: a shared subsurface asset, in urgent need of sound governance |
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Book Chapter |
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Year |
2021 |
Publication |
Global Groundwater |
Abbreviated Journal |
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113-128 |
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ILC Draft Articles, impact on GDP, sound governance, Transboundary aquifers |
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Apart from some notable exceptions, the sound governance of transboundary aquifers (coupled or uncoupled to rivers) is seriously lacking in most regions of the world, despite a highly successful 20-year ISARM initiative. The distinction between regions of water abundance (as in the Haute Savoie–Geneva aquifers) and those of water scarcity (\textless1000 m3/an/capita), as in the Rum-Saq aquifer, ought to be a driver for the urgency in adopting sound governance. In the latter regions, however, such an urgent response faces too many hurdles (institutional, financial, and weak capacity). Climate change, one of the global megatrends (among demography, economic shift, resources stress, urbanization, and novel viruses such as COVID-19), will exacerbate the problem in the coming decade and beyond. This chapter provides an critical perspective on the status of this subsurface asset in 570 or so, domestic and transboundary aquifers of the world (self-identified by country experts), while taking full account of their interconnections, or not, with surface waters. This critical perspective will be grounded in two important factors, first the hiatus in adoption by countries of the evolving international water law and guidance on transboundary aquifers (the Draft Articles, which provide legal pathways for collaboration or eventually dispute resolution), and second the framework of the sustainable development goals (SDG) 6 (clean water and sanitation), which countries have committed themselves to with reference to transboundary waters. The critical perspective finds that despite the lack of momentum in adopting formal global norms, sporadic cooperation and collaboration is continuing and is well received, when delivered methodically through the support of international agencies. The findings of the critical perspective are that even if water-related SDGs will have been achieved across the world, it would contribute precious little to meaningful enhancement of governance of transboundary aquifers, unless they have been explicitly addressed in terms that are tangible to decision makers, such as the impact of disregarding them on the current or future national GDP. The onset of a “new socioeconomic normal” in the aftermath of COVID-19 could further defer meaningful progress, taking the example of Latin America, where a 5% decline has been forecast for 2020. With such declines in the finances of governments, attention to shared aquifer resources may well decline even further. Urgent wise reaction to this possibility must be a priority for the professional science-policy community. |
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Elsevier |
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Mukherjee, A.; Scanlon, B.R.; Aureli, A.; Langan, S.; Guo, H.; McKenzie, A.A. |
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978-0-12-818172-0 |
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THL @ christoph.kuells @ mukherjee_chapter_2021 |
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106 |
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Bonnetti, C.; Zhou, L.; Riegler, T.; Brugger, J.; Fairclough, M. |
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Title |
Large S isotope and trace element fractionations in pyrite of uranium roll front systems result from internally-driven biogeochemical cycle |
Type |
Journal Article |
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Year |
2020 |
Publication |
Geochimica et Cosmochimica Acta |
Abbreviated Journal |
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Volume |
282 |
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Pages |
113-132 |
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Keywords |
Activity cycle, Pyrite composition, Roll front uranium deposits, S isotope and trace element fractionation |
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Abstract |
Complex pyrite textures associated with large changes in isotopic and trace element compositions are routinely assumed to be indicative of multi-faceted processes involving multiple fluid and sulfur sources. We propose that the features of ore-stage pyrite from roll front deposits across the world, revealed in exquisite detail via high-resolution trace element mapping by LA-ICP-MS, reflect the dynamic internal evolution of the biogeochemical processes responsible for sulfate reduction, rather than externally driven changes in fluid or sulfur sources through time. Upon percolation of oxidizing fluids into the reduced host-sandstones, roll front systems become self-organized, with a systematic reset of their activity cycle after each translation stage of the redox interface down dip of the aquifer. Dominantly reducing conditions at the redox interface favor the formation of biogenic framboidal pyrite (δ34S from −30.5 to −12.5‰) by bacterial sulfate reduction and the genesis of the U mineralization. As the oxidation front advances, oxidation of reduced sulfur minerals induces an increased supply of sulfate and metals in solution to the bacterial sulfate reduction zone that has similarly advanced down the flow gradient. Hence, this stage is marked by increased rates of the bacterial sulfate reduction associated with the crystallization of variably As-Co-Ni-Mo-enriched concentric pyrite (up to 10,000′s of ppm total trace contents) with moderately negative δ34S values (from −13.7 to −7.5‰). A final stage of pyrite cement with low trace element contents and heavier δ34S signature (from −6.9 to +18.8‰) marks the end of the roll front activity cycle and the transition from an open to a predominantly closed system behavior (negligible advection of fresh sulfate). Blocky pyrite cement is formed using the remaining sulfate, which now becomes quickly heavy according to a Rayleigh isotope fractionation process. This ends the cycle by depleting the nutrient supplies for the sulfate-reducing bacteria and cementing pore spaces within the host sandstone, effectively restricting fluid infiltration. This internally-driven roll front activity cycle results in systematic, large S isotope and trace element fractionation. Ultimately, the long-time evolution of the basin and fluid sources control the metal endowment and evolution of the system; these events, however, are unlikely to be preserved by the roll front, as a direct result of its hydrodynamic nature. |
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0016-7037 |
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THL @ christoph.kuells @ bonnetti_large_2020 |
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185 |
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Author |
Karaimeh, S.A. |
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Title |
Maintaining desert cultivation: Roman, Byzantine, and Early Islamic water-strategies at Udhruh region, Jordan |
Type |
Journal Article |
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Year |
2019 |
Publication |
Journal of Arid Environments |
Abbreviated Journal |
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166 |
Issue |
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Pages |
108-115 |
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Keywords |
Irrigation, Qanat, Cultivation, Arid environment, Nabataean, Jordan |
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Abstract |
The site of Udhruh is located in the arid desert of southern Jordan, about 15 km to the east of Petra. The site was built by the Nabataeans but expanded by the Romans (as a defensive site) and was continuously occupied until the Early Islamic period. It receives less than the 200 mm of annual precipitation, which is crucial for agricultural cultivation. Archaeological evidence from earlier excavations together with new data from several survey projects indicate that areas around Udhruh were cultivated throughout the Roman, Byzantine, and Early Islamic periods (300 BCE–800 CE). The fundamental question is: how did the people of Udhruh sustain their community in the desert, and how did they transform the desert into arable land? The landscape could be utilised thanks to sophisticated water management and irrigation techniques. At least four underground qanat systems were identified providing Udhruh with access to groundwater. At the terminal end of the qanat systems, several types of closed surface channels conveyed the water to reservoirs, which subsequently distributed the water to the field systems. The water systems of Udhruh differ from the well-known Nabataean systems in the surrounding area. As Udhruh was taken over by the Roman army in 106 CE, this study analyses how the Nabataean water systems continued to function and adapt through the Roman and Byzantine periods. A complete understanding of Udhruh’s water systems helps to reconstruct past land use, agricultural activity, and irrigation practices in a currently arid region. |
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0140-1963 |
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THL @ christoph.kuells @ Alkaraimeh2019108 |
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271 |
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Klaus, J.; Zehe, E.; Elsner, M.; Külls, C.; McDonnell, J.J. |
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Title |
Macropore flow of old water revisited: experimental insights from a tile-drained hillslope |
Type |
Journal Article |
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Year |
2013 |
Publication |
Hydrology and Earth System Sciences |
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17 |
Issue |
1 |
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103 |
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Copernicus GmbH |
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THL @ christoph.kuells @ Klaus2013macropore |
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23 |
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Author |
Chase, B.M.; Meadows, M.E. |
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Title |
Late Quaternary dynamics of southern Africa’s winter rainfall zone |
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Journal Article |
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Year |
2007 |
Publication |
Earth-Science Reviews |
Abbreviated Journal |
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84 |
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3 |
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103-138 |
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Last Glacial Maximum, palaeoenvironment, Quaternary, southern Africa, westerlies, winter rainfall zone |
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Abstract |
Variations in the nature and extent of southern Africa’s winter rainfall zone (WRZ) have the potential to provide important information concerning the nature of long-term climate change at both regional and hemispheric scales. Positioned at the interface between tropical and temperate systems, southern Africa’s climate is influenced by shifts in the Intertropical Convergence Zone, the westerlies, and the development and position of continental and oceanic anticyclones. Over the last glacial–interglacial cycle substantial changes in the amount and seasonality of precipitation across the subcontinent have been linked to the relative dominance of these systems. Central to this discussion has been the extent to which the region’s glacial climates would have been affected by expansions of Antarctic sea-ice, equatorward migrations of the westerlies, more frequent/intense winter storms and an expanded WRZ. This paper reviews the developing body of evidence pertaining to shifts in the WRZ, and the evolution of ideas that have been presented to explain the patterns observed. Dividing the region into three separate axes, along the western and southern margins of the continent and across the interior into the Karoo and the Kalahari, a range of evidence from both terrestrial sites and marine cores is considered, and potential expansions of the WRZ expansions are explored. Despite the limitations of many of the region’s proxy records, a coherent pattern has begun to develop of a significantly expanded WRZ during phases of the last glacial period, with the best-documented being between 32–17 ka. While more detailed inferences will require the recovery and analysis of longer and better-dated records, this synthesis provides a new baseline for further research in this key region. |
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0012-8252 |
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THL @ christoph.kuells @ chase_late_2007 |
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102 |
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Bullock, L.A.; Parnell, J. |
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Title |
Selenium and molybdenum enrichment in uranium roll-front deposits of Wyoming and Colorado, USA |
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Journal Article |
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Year |
2017 |
Publication |
Journal of Geochemical Exploration |
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180 |
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101-112 |
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Keywords |
Molybdenum, Roll-fronts, Selenium, Tellurium, Uranium, Wyoming |
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Abstract |
Sandstone uranium (U) roll-front deposits of Wyoming and Colorado (USA) are important U resources, and may provide a terrestrial source for critical accessory elements, such as selenium (Se), molybdenum (Mo), and tellurium (Te). Due to their associated toxicity, MoSeTe occurrences in roll-fronts should also be carefully monitored during U leaching and ore processing. While elevated MoSe concentrations in roll-fronts are well established, very little is known about Te occurrence in such deposits. This study aims to establish MoSeTe concentrations in Wyoming and Colorado roll-fronts, and assess the significance of these deposits in an environmental and mineral exploration context. Sampled roll-front deposits, produced by oxidized groundwater transportation through a sandstone, show high MoSe content in specific redox zones, and low Te, relative to crustal means. High Se concentrations (up to 168ppm) are restricted to a narrow band of alteration at the redox front. High Mo content (up to 115ppm) is typically associated with the reduced mineralized nose and seepage zones of the roll-front, ahead of the U orebody. Elevated trace element concentrations are likely sourced from proximal granitic intrusions, tuffaceous deposits, and local pyritic mudstones. Elevated MoSe content in the sampled roll fronts may be regarded as a contaminant in U in-situ recovery and leaching processing, and may pose an environmental threat in groundwaters and soils, so extraction should be carefully monitored. The identification of peak concentrations of MoSe can also act as a pathfinder for the redox front of a roll-front, and help to isolate the U orebody, particularly in the absence of gamma signatures. |
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0375-6742 |
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THL @ christoph.kuells @ bullock_selenium_2017 |
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189 |
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Tan, K.; Li, C.; Liu, J.; Qu, H.; Xia, L.; Hu, Y.; Li, Y. |
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A novel method using a complex surfactant for in-situ leaching of low permeable sandstone uranium deposits |
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Journal Article |
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2014 |
Publication |
Hydrometallurgy |
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150 |
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99-106 |
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Complex surfactant, In-situ leaching of uranium mining, Leaching kinetics, Low permeable sandstone uranium deposit, Resin adsorption and elution |
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Applications of a complex surfactant developed in-house to in-situ leaching of low permeable sandstone uranium deposits are described based on results from agitation leaching, column leaching, resin adsorption, and elution experiments using uranium containing solution from the in-situ leaching site. The results of agitation leaching experiments show that adding surfactant with different concentrations into leaching solution improves the leaching rate of uranium. The maximum leaching rate of uranium from agitation leaching reached 92.6% at an added surfactant concentration of 10mg/l. Result of column leaching experiment shows that adding surfactant with varying concentrations into leaching solutions increased the permeability coefficient of ore-bearing layer by 42.7–86.8%. The leaching rate of uranium from column leaching increased by 58.0% and reached 85.8%. The result of kinetic analysis shows that for the extraction of uranium controlled by diffusion without surfactant the apparent rate constant 0.0023/d changed to 0.0077/d for the extraction with surfactant controlled by both diffusion and surface chemical reactions. Results from resin adsorption and elution experiments show that there was no influence on resin adsorption and elution of uranium with an addition of 50mg/l surfactant to production solution from in-situ leaching. The adsorption curve, sorption capacity of resin, recycling of resin remained the same as without adding any surfactant. Introducing complex surfactant to leaching solution increased the peak concentration of uranium in eluents, reduced the residual uranium content in resin, and promoted the elution efficiency. The method of using a complex surfactant for in-situ leaching is useful for low permeable sandstone uranium deposits. |
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0304-386x |
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THL @ christoph.kuells @ tan_novel_2014 |
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201 |
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Demuth, S.; Külls, C. |
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Probability analysis and regional aspects of droughts in southern Germany |
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1997 |
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Sustainability of Water Resources under Increasing Uncertainty |
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240 |
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97 |
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Iahs |
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THL @ christoph.kuells @ Demuth1997probability |
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35 |
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Pereira, A.J.S.C.; Neves, L.J.P.F. |
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Estimation of the radiological background and dose assessment in areas with naturally occurring uranium geochemical anomalies—a case study in the Iberian Massif (Central Portugal) |
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Journal Article |
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2012 |
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Journal of Environmental Radioactivity |
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112 |
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96-107 |
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Background, Dose assessment, Geochemical anomalies, Mine remediation, Natural radioactivity, Uranium |
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Naturally occurring uranium geochemical anomalies, representative of the several thousand recognized in the Portuguese section of the Iberian Massif and outcropping in three target areas with a total of a few thousand square metres, were subjected to a detailed study (1:1000 scale) to evaluate the radiological health-risk on the basis of a dose assessment. To reach this goal some radioactive isotopes from the uranium, thorium and potassium radioactive series were measured in 52 samples taken from different environmental compartments: soils, stream sediments, water, foodstuff (vegetables) and air; external radiation was also measured through a square grid of 10×10m, with a total of 336 measurements. The results show that some radioisotopes have high activities in all the environmental compartments as well as a large variability, namely for those of the uranium decay chain, which is a common situation in the regional geological setting. Isotopic disequilibrium is also common and led to an enrichment of several isotopes in the different pathways, as is the case of 226Ra; maximum values of 1.76BqL−1 (water), 986Bqkg−1 (soils) and 18.9Bqkg−1 (in a turnip sample) were measured. On the basis of a realistic scenario combined with the experimental data, the effective dose from exposure to ionizing radiation for two groups of the population (rural and urban) was calculated; the effective dose is variable between 8.0 and 9.5mSvyear−1, which is 3–4 times higher than the world average. Thus, the radiological health-risk for these populations could be significant and the studied uranium anomalies must be taken into account in the assessment of the geochemical background. The estimated effective dose can also be used as typical of the background of the Beiras uranium metalogenetic province and therefore as a “benchmark” in the remediation of the old uranium mining sites. |
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0265-931x |
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THL @ christoph.kuells @ pereira_estimation_2012 |
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129 |
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Akter, A.; Tanim, A.H.; Islam, M.K. |
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Possibilities of urban flood reduction through distributed-scale rainwater harvesting |
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Journal Article |
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2020 |
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Water Science and Engineering |
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13 |
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2 |
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95-105 |
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Low-impact development (LID), SWMM, HEC-RAS, Remote sensing, Urban flooding, Inundation depth |
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Urban flooding in Chittagong City usually occurs during the monsoon season and a rainwater harvesting (RWH) system can be used as a remedial measure. This study examines the feasibility of rain barrel RWH system at a distributed scale within an urbanized area located in the northwestern part of Chittagong City that experiences flash flooding on a regular basis. For flood modeling, the storm water management model (SWMM) was employed with rain barrel low-impact development (LID) as a flood reduction measure. The Hydrologic Engineering Center’s River Analysis System (HEC-RAS) inundation model was coupled with SWMM to observe the detailed and spatial extent of flood reduction. Compared to SWMM simulated floods, the simulated inundation depth using remote sensing data and the HEC-RAS showed a reasonable match, i.e., the correlation coefficients were found to be 0.70 and 0.98, respectively. Finally, using LID, i.e., RWH, a reduction of 28.66% could be achieved for reducing flood extent. Moreover, the study showed that 10%–60% imperviousness of the subcatchment area can yield a monthly RWH potential of 0.04–0.45 m3 from a square meter of rooftop area. The model can be used for necessary decision making for flood reduction and to establish a distributed RWH system in the study area. |
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1674-2370 |
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THL @ christoph.kuells @ Akter202095 |
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247 |
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