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Smedley, P.L.; Bearcock, J.M.; Ward, R.S.; Crewdson, E.; Bowes, M.J.; Darling, W.G.; Smith, A.C. |
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Title |
Monitoring of methane in groundwater from the Vale of Pickering, UK: Temporal variability and source discrimination |
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Journal Article |
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Year |
2023 |
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Chemical Geology |
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636 |
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121640 |
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Aquifer, Biogenic, Ethane, Hydrocarbons, Methane, Shale gas |
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Groundwater abstracted from aquifers in the Vale of Pickering, North Yorkshire, UK and monitored over the period 2015–2022, shows evidence of variable but commonly high concentrations of dissolved CH4. Sampled groundwater from the Jurassic organic-rich Kimmeridge Clay Formation (boreholes up to 180 m depth) has concentrations up to 57 mg/L, and concentrations up to 59 mg/L are found in groundwater from underlying confined Corallian Group limestone (borehole depths 50–227 m). The high concentrations are mainly from boreholes in the central parts of the vale. Small concentrations of ethane (C2H6, up to 800 μg/L) have been found in the Kimmeridge Clay and confined Corallian groundwaters, and of propane (C3H8, up to 160 μg/L) in deeper boreholes (110–180 m) from these formations. The concentrations are typically higher in groundwater from the deeper boreholes and vary with hydrostatic pressure, reflecting the pressure control on CH4 solubility. The occurrences contrast with groundwater from shallow Quaternary superficial deposits which have low CH4 concentrations (up to 0.39 mg/L), and with the unconfined and semi-confined sections of the Corallian aquifer (up to 0.7 mg/L) around the margins of the vale. Groundwater from the Quaternary, Kimmeridge Clay formations and to a small extent the confined Corallian aquifer, supports local private-water supplies, that from the peripheral unconfined sections of Corallian also supports public supply for towns and villages across the region. Dissolved methane/ethane (C1/C2) ratios and stable-isotopic compositions (δ13C-CH4, δ2H-CH4 and δ13C-CO2) suggest that the high-CH4 groundwater from both the Kimmeridge Clay and confined Corallian formations derives overwhelmingly from biogenic reactions, the methanogenesis pathway by CO2 reduction. A small minority of groundwater samples shows a more enriched δ13C-CH4 composition (−50 to −44 ‰) which has been interpreted as due to anaerobic or aerobic methylotrophic oxidation in situ or post-sampling oxidation, rather than derivation by a thermogenic route. Few of the existing groundwater sites are proximal to abandoned or disused conventional hydrocarbon wells that exist in the region, and little evidence has been found for an influence on groundwater dissolved gases from these sites. The Vale of Pickering has also been under recent consideration for development of an unconventional hydrocarbon (shale-gas) resource. In this context, the monitoring of dissolved gases has been an important step in establishing the high-CH4 baseline of groundwaters from Jurassic deposits in the region and in apportioning their sources and mechanisms of genesis. |
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0009-2541 |
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THL @ christoph.kuells @ smedley_monitoring_2023 |
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172 |
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Etschmann, B.; Liu, W.; Li, K.; Dai, S.; Reith, F.; Falconer, D.; Kerr, G.; Paterson, D.; Howard, D.; Kappen, P.; Wykes, J.; Brugger, J. |
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Title |
Enrichment of germanium and associated arsenic and tungsten in coal and roll-front uranium deposits |
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Journal Article |
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2017 |
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Chemical Geology |
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463 |
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29-49 |
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Arsenic, Coal, EXAFS and XANES, germanium, Hydrothermal fluids, Metallogenesis, Speciation, Tungsten |
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Most of the World’s germanium (Ge) is mined from Ge-rich lignite, where it is commonly associated with elevated arsenic (As), tungsten (W) and beryllium (Be) contents. Over the past decade, new evidence showing that World-class Ge deposits result from the interaction of hydrothermal fluids with organic matter in coal seams has emerged. Yet, the chemical state of Ge and associated metals in lignite remains poorly understood. We used Mega-pixel Synchrotron X-ray Fluorescence (MSXRF), X-ray Absorption Near Edge Structure (XANES) and Extended X-ray Absorption Fine Structure (EXAFS) to characterize the oxidation states and chemical bonding environment of Ge, As, and W in two world-class Mesozoic Ge-in-lignite deposits (Lincang, Yunnan, southwestern China; Wulantuga, Inner Mongolia, northeastern China); in lignite-bearing uranium (U) ores from the Beverley deposit (South Australia) hosted in Eocene sandstones; and in lignite and preserved wood in late Oligocene-Miocene fluviatile sediments (Gore, Southland, New Zealand). The aim was to improve our understanding of the enrichment mechanism of Ge in lignite and better evaluate the environmental mobility of Ge and some of the associated metals (specifically As and W) in lignite ores. In all samples, chemical maps show that Ge is distributed homogeneously (down to 2μm) within the organic matter. XANES and EXAFS data show that Ge exists in the tetravalent oxidation state and in a distorted octahedral coordination with O, consistent with complexing of Ge by organic ligands. In some pyrite-bearing samples, a minor fraction of Ge is also present as Ge(IV) in association with pyrite. In contrast, As displays a more complex speciation pattern, sometimes even in a single sample, including As(III), As(V), and As(−I/+II) in solid solution in sulfides. Arsenic in sulfides occurs in anionic and cationic forms, i.e., it shows both the common substitution for S22− and the substitution for Fe recently discovered in some hydrothermal pyrites. Tungsten was present as W(VI) in distorted octahedral (3+3) coordination. The EXAFS data confirm the absence or minor contribution of individual W-rich minerals such as scheelite or ferberite to W mass balance in the studied samples. These data show that Ge, W, and probably some As are scavenged via formation of insoluble, oxygen-bridged metal organic complexes in lignite. Destruction of the organic ligands responsible for fixing Ge and W (As) in these lignites is required for liberating the metals, e.g. from waste materials. Geochemical modelling suggests that Ge, W, Be and As all can be extracted from granitic rocks by dilute, low temperature hydrothermal fluids. Germanium is transported mainly as the tetrahedral Ge(OH)4(aq) complex, but fixed as an octahedral oxy-bridged organic complex. The same situation is valid for W, which is transported at the tetrahedral tungstate ion, but most likely scavenged via formation of a 6-coordinated metal-organic species. The Ge-Be-W±As association in Ge-rich coals reflects the source of the metals as well as related scavenging mechanisms. |
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THL @ christoph.kuells @ etschmann_enrichment_2017 |
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183 |
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Illgen, M.; Ackermann, H. |
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2019 |
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Urban Flood Prevention: Technical and Institutional Aspects from Chinese and German Perspective |
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173-193 |
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Today’s cities face the challenge of climate change adaptation worldwide. In this context, prevention of damage caused by flash floods plays an important role. This requires a cooperative pluvial flood risk management approach, which includes planning, technical, and administrative measures and involves preliminary flood risk analyses. This article outlines the main components of this risk management approach, which has proven its effectiveness in Europe. The recommendations formulated for this purpose are applicable or adaptable to regions with other constraints, such as China, for example. |
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Springer International Publishing |
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Cham |
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Köster, S.; Reese, M.; Zuo, J.’e |
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978-3-030-01488-9 |
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THL @ christoph.kuells @ Illgen2019 |
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87 |
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Severi, A.; Masoudian, M.; Kordi, E.; Roettcher, K. |
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Discharge coefficient of combined-free over-under flow on a cylindrical weir-gate |
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2015 |
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ISH Journal of Hydraulic Engineering |
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21 |
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1 |
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42-52 |
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Taylor & Francis |
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THL @ christoph.kuells @ doi:10.1080/09715010.2014.939503 |
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88 |
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de Jong, I.J.H.; Arif, S.S.; Gollapalli, P.K.R.; Neelam, P.; Nofal, E.R.; Reddy, K.Y.; Röttcher, K.; Zohrabi, N. |
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Improving agricultural water productivity with a focus on rural transformation* |
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2021 |
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Irrigation and Drainage |
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70 |
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3 |
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458-469 |
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irrigation efficiency, water productivity, rural transformation, efficacité de l’irrigation, productivité de l’eau, transformation rurale |
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ABSTRACT As a result of population growth, economic development and climate change, feeding the world and providing water security will require important changes in the technologies, institutions, policies and incentives that drive present-day water management, as captured in Goal 6.4 of the Millennium Development Goals. Irrigation is the largest and most inefficient water user, and there is an expectation that even small improvements in agricultural water productivity will improve water security. This paper argues that improvements in irrigation water productivity involves a complex and comprehensive rural transformation that goes beyond mere promotion of water saving technologies. Many of the measures to improve water productivity require significant changes in the production systems of farmers and in the support provided to them. Looking forward, water use and competition over water are expected to further increase. By 2025, about 1.8 billion people will be living in regions or countries with absolute water scarcity. Demand for water will rise exponentially, while supply becomes more erratic and uncertain, prompting the need for significant shifts of inter-sectoral water allocation to support continued economic growth. Advances in the use of remote sensing technologies will make it increasingly possible to cost-effectively and accurately estimate crop evapotranspiration from farmers’ fields. |
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THL @ christoph.kuells @ https://doi.org/10.1002/ird.2451 |
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89 |
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Röttcher, K. |
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2018 |
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Risikomanagement und Nachhaltigkeit in der Wasserwirtschaft: Erfolgreiche Navigation durch die Komplexität und Dynamik des Risikos |
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165-174 |
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Im vorliegenden Beitrag werden beispielhaft unterschiedliche Ansätze des Risikomanagements und das Verständnis von Nachhaltigkeit in der Wasserwirtschaft dargelegt. Die Darstellung richtet sich insbesondere an Leser aus anderen Fachdisziplinen, wie das Rechts- und Finanzwesen, den Fahrzeug- und Maschinenbau oder auch die sozialen Berufe. Die Zusammenhänge werden überblicksartig mit einzelnen konkreten Beispielen dargestellt mit dem Fokus auf die grundsätzlichen Denk- und Vorgehensweisen. |
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Springer Fachmedien Wiesbaden |
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Wiesbaden |
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Michalke, A.; Rambke, M.; Zeranski, S. |
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978-3-658-19684-4 |
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THL @ christoph.kuells @ Röttcher2018 |
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90 |
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Wolfe, P. |
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Title |
The Simplex Method For Quadratic Programming |
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1959 |
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Econometrica |
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170 |
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THL @ christoph.kuells @ Wolfe1959 |
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285 |
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United Nations |
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Stampriet Transboundary Aquifer System Assessment: governance of Groundwater resources in Transboundary Aquifers (GGRETA), phase 1: technical report |
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1998 |
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Incl. bibl. |
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THL @ christoph.kuells @ |
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286 |
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Zwartendijk, B.W.; Ghimire C. P.; Ravelona M.; Lahitiana J.; van Meerveld H. J. |
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Hydrometric data and stable isotope data for streamflow and rainfall in the Marolaona catchment, Madagascar, 2015-2016 |
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Miscellaneous |
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2023 |
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NERC EDS Environmental Information Data Centre |
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THL @ christoph.kuells @ ref10.5285/f93d87ed-7bc4-4d03-9690-3856e6cbbd11 |
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289 |
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Author |
Puri, S. |
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Chapter 9 – Transboundary aquifers: a shared subsurface asset, in urgent need of sound governance |
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2021 |
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Global Groundwater |
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113-128 |
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ILC Draft Articles, impact on GDP, sound governance, Transboundary aquifers |
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Apart from some notable exceptions, the sound governance of transboundary aquifers (coupled or uncoupled to rivers) is seriously lacking in most regions of the world, despite a highly successful 20-year ISARM initiative. The distinction between regions of water abundance (as in the Haute Savoie–Geneva aquifers) and those of water scarcity (\textless1000 m3/an/capita), as in the Rum-Saq aquifer, ought to be a driver for the urgency in adopting sound governance. In the latter regions, however, such an urgent response faces too many hurdles (institutional, financial, and weak capacity). Climate change, one of the global megatrends (among demography, economic shift, resources stress, urbanization, and novel viruses such as COVID-19), will exacerbate the problem in the coming decade and beyond. This chapter provides an critical perspective on the status of this subsurface asset in 570 or so, domestic and transboundary aquifers of the world (self-identified by country experts), while taking full account of their interconnections, or not, with surface waters. This critical perspective will be grounded in two important factors, first the hiatus in adoption by countries of the evolving international water law and guidance on transboundary aquifers (the Draft Articles, which provide legal pathways for collaboration or eventually dispute resolution), and second the framework of the sustainable development goals (SDG) 6 (clean water and sanitation), which countries have committed themselves to with reference to transboundary waters. The critical perspective finds that despite the lack of momentum in adopting formal global norms, sporadic cooperation and collaboration is continuing and is well received, when delivered methodically through the support of international agencies. The findings of the critical perspective are that even if water-related SDGs will have been achieved across the world, it would contribute precious little to meaningful enhancement of governance of transboundary aquifers, unless they have been explicitly addressed in terms that are tangible to decision makers, such as the impact of disregarding them on the current or future national GDP. The onset of a “new socioeconomic normal” in the aftermath of COVID-19 could further defer meaningful progress, taking the example of Latin America, where a 5% decline has been forecast for 2020. With such declines in the finances of governments, attention to shared aquifer resources may well decline even further. Urgent wise reaction to this possibility must be a priority for the professional science-policy community. |
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Elsevier |
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Mukherjee, A.; Scanlon, B.R.; Aureli, A.; Langan, S.; Guo, H.; McKenzie, A.A. |
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978-0-12-818172-0 |
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THL @ christoph.kuells @ mukherjee_chapter_2021 |
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106 |
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