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Pree, T.A.D. |
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Title |
The politics of baselining in the Grants uranium mining district of northwestern New Mexico |
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Journal Article |
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Year |
2020 |
Publication |
Journal of Environmental Management |
Abbreviated Journal |
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268 |
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110601 |
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Critical stakeholder analysis, Environmental cleanup, Environmental monitoring, Mining reclamation/remediation/restoration, Politics of baselining |
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During the second half of the twentieth century, northwestern New Mexico served as the primary production site for one of the world’s largest nuclear arsenals. From 1948 to 1970 the “Grants uranium district” provided almost half of the total uranium ore accumulated by the United States federal government for the production of nuclear weapons, in addition to becoming a national source for commercial nuclear energy from the late 1960s to the early 1990s. By the twenty-first century, after a prolonged period of economic decline that began in the late 1970s, all uranium mining and milling in New Mexico had ceased, leaving a legacy of environmental health impacts. What was once referred to as “The Uranium Capital of the World” now encompasses over a thousand abandoned uranium mines and seven massive uranium mill tailings piles, which are associated with airborne and soil contamination as well as groundwater plumes of uranium and other contaminants of concern, in a landscape that has been fractured by underground mine workings and punctured by thousands of exploratory boreholes. This article presents an ethnographic study of the diverse forms of expertise involved in monitoring and managing the mine waste and mill tailings. Drawing from over two years of ethnographic research, I describe the relationship between different stakeholders from local communities, government agencies, and transnational mining corporations as they deliberate about the possibility of cleaning up the former mining district. My thesis is that the possibility of cleaning up the Grants district hinges on the “politics of baselining”—a term I introduce to describe the relationship between stakeholders and their competing environmental models and hydrogeological theories; each accounts for a different geological past prior to mining that can be deemed “natural,” as the background against which to measure the anthropogenic impacts from mining. |
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0301-4797 |
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THL @ christoph.kuells @ pree_politics_2020 |
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151 |
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Gimeno, M.J.; Tullborg, E.-L.; Nilsson, A.-C.; Auqué, L.F.; Nilsson, L. |
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Title |
Hydrogeochemical characterisation of the groundwater in the crystalline basement of Forsmark, the selected area for the geological nuclear repositories in Sweden |
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Journal Article |
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Year |
2023 |
Publication |
Journal of Hydrology |
Abbreviated Journal |
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624 |
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129818 |
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Crystalline bedrock, Deep geological repository, Glacial meltwater intrusion, Groundwater mixing, Hydrogeochemical model, Nuclear waste disposal |
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Numerous groundwater analyses from the crystalline bedrock in the Forsmark area have been performed between 2002 and 2019, together with thorough geological, geophysical, and hydrogeological studies, within the site investigations carried out by the Swedish Nuclear Fuel and Waste Management Company. The groundwater samples have been taken from boreholes down to ≈ 1000 m and the analysis include major- and trace-elements, stable and radiogenic isotopes, gases and microbes. The chemical and isotopic composition of these groundwaters evidences the presence of non-marine brackish to saline groundwaters with very long residence times (many hundreds of thousands of years) and a series of complex mixing events resulting from the recharge of different waters over time: glacial meltwaters, probably from different glaciations of which the latest culminated some 20,000 years ago, and marine waters from the Baltic starting some 7000 years ago. Later, meteoric water and present Baltic Sea water have recharged in different parts of the upper 100 m. These mixing events have also triggered chemical and microbial reactions that have conditioned some of the important groundwater parameters and, together with the structural complexity of the area, they have promoted a heterogeneous distribution of groundwater compositions in the bedrock. Due to these evident differences in chemistry, residence time and origin of the groundwater, several groundwater types were defined in order to facilitate the visualisation and communication. The differentiation (linked to the paleohydrological history of the area) was based on Cl concentration, Cl/Mg ratio (marine component), and δ18O value (glacial component). The work presented in this paper increases the understanding of the groundwater evolution in fractured and compartmentalised aquifers where mixing processes are the most important mechanisms. The model proposed to characterise the present groundwater system of the Forsmark area will also help to predict the future hydrogeochemical behaviour of the groundwater system after the construction of the repositories for the nuclear wastes. |
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0022-1694 |
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THL @ christoph.kuells @ gimeno_hydrogeochemical_2023 |
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137 |
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Ammar, F.H.; Deschamps, P.; Chkir, N.; Zouari, K.; Agoune, A.; Hamelin, B. |
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Title |
Uranium isotopes as tracers of groundwater evolution in the Complexe Terminal aquifer of southern Tunisia |
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Journal Article |
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Year |
2020 |
Publication |
Quaternary International |
Abbreviated Journal |
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547 |
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33-49 |
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CT southern Tunisia, Holocene, Mixing, Radicarbon, Uranium isotopes, Water-rock interaction |
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The Complexe Terminal (CT) multi-layer aquifer is formed by Neogene/Paleogene sand deposits, Upper Senonian (Campanian-Maastrichtian limestones) and Turonian carbonates. The chemical composition and isotopes of carbon and uranium were investigated in groundwater sampled from the main hydrogeological units of the (CT) aquifer in southern Tunisia. We paid special attention to the variability of uranium contents and isotopes ratio (234U/238U) to provide a better understanding of the evolution of the groundwater system. Uranium concentrations range from 1.5 to 19.5 ppb, typical of oxic or mildly reducing conditions in groundwaters. The lowest concentrations are found southeast of the study area, where active recharge is supposed to take place. When looking at the isotope composition, it appears that all the samples, including those from carbonate levels, are in radioactive disequilibrium with significant 234U excess. A clear-cut distinction is observed between Turonian and Senonian carbonate aquifers on the one hand, with 234U/238U activity ratios between 1.1 and 1.8, and the sandy aquifer on the other hand, showing higher ratios from 1.8 to 3.2. The distribution of uranium in this complex aquifer system seems to be in agreement with the lithological variability and are ultimately a function of a number of physical and chemical factors including the uranium content of the hosting geological formation, water-rock interaction and mixing between waters having different isotopic signatures. Significant relationships also appear when comparing the uranium distribution with the major ions composition. It is noticeable that uranium is better correlated with sulfate, calcium and magnesium than with other major ions as chloride or bicarbonate. The 14C activities and δ13C values of DIC cover a wide range of values, from 1.1 pmc to 30.2 pmc and from −3.6‰ to −10.7‰, respectively. 14C model ages estimated by the Fontes and Garnier model are all younger than 22 Ka and indicate that the recharge of CT groundwater occurred mainly during the end of the last Glacial and throughout the Holocene. |
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1040-6182 |
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THL @ christoph.kuells @ ammar_uranium_2020 |
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119 |
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Paradis, C.J.; Hoss, K.N.; Meurer, C.E.; Hatami, J.L.; Dangelmayr, M.A.; Tigar, A.D.; Johnson, R.H. |
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Title |
Elucidating mobilization mechanisms of uranium during recharge of river water to contaminated groundwater |
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Journal Article |
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Year |
2022 |
Publication |
Journal of Contaminant Hydrology |
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251 |
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Pages |
104076 |
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Keywords |
Desorption, Dissolution, Groundwater, Surface water, Tracer, Uranium |
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The recharge of stream water below the baseflow water table can mobilize groundwater contaminants, particularly redox-sensitive and sorptive metals such as uranium. However, in-situ tracer experiments that simulate the recharge of stream water to uranium-contaminated groundwater are lacking, thus limiting the understanding of the potential mechanisms that control the mobility of uranium at the field scale. In this study, a field tracer test was conducted by injecting 100 gal (379 l) of oxic river water into a nearby suboxic and uranium-contaminated aquifer. The traced river water was monitored for 18 days in the single injection well and in the twelve surrounding observation wells. Mobilization of uranium from the solid to the aqueous phase was not observed during the tracer test despite its pre-test presence being confirmed on the aquifer sediments from lab-based acid leaching. However, strong evidence of oxidative immobilization of iron and manganese was observed during the tracer test and suggested that immobile uranium was likely in its oxidized state as U(VI) on the aquifer sediments; these observations ruled out oxidation of U(IV) to U(VI) as a potential mobilization mechanism. Therefore, desorption of U(VI) appeared to be the predominant potential mobilization mechanism, yet it was clearly not solely dependent on concentration as evident when considering that uranium-poor river water (\textless0.015 mg/L) was recharged to uranium-rich groundwater (≈1 mg/L). It was possible that uranium desorption was limited by the relatively higher pH and lower alkalinity of the river water as compared to the groundwater; both factors favor immobilization. However, it was likely that the immobile uranium was associated with a mineral phase, as opposed to a sorbed phase, thus desorption may not have been possible. The results of this field tracer study successfully ruled out two common mobilization mechanisms of uranium: (1) oxidative dissolution and (2) concentration-dependent desorption and ruled in the importance of advection, dispersion, and the mineral phase of uranium. |
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0169-7722 |
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THL @ christoph.kuells @ paradis_elucidating_2022 |
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135 |
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Petisco-Ferrero, S.; Idoeta, R.; Rozas, S.; Olondo, C.; Herranz, M. |
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Radiological environmental monitoring of groundwater around NPP: A proposal for its assessment |
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Journal Article |
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Year |
2023 |
Publication |
Heliyon |
Abbreviated Journal |
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9 |
Issue |
9 |
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19470 |
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Detection limit, Nuclear power plant dismantling and decommissioning, Radiological environmental monitoring, Radionuclides in groundwater |
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Whether a nuclear installation has radiological impact and, in that case, its extension, are the questions behind any environmental analysis of the installation along its operational life. This analysis is based on the detailed establishment of the radiological background of the area. Accordingly, the dismantling and decommissioning process (D&D) of a nuclear power plant starts with a radiological monitoring plan, which includes the radiological characterization of the area and of its surroundings. At the completion of the D&D, unrestricted use for the site will be permitted strictly in accordance with results of the radiological survey within the limits established by the local authorities. Groundwater quality is typically included in any radiological analysis since, among other reasons, a significant part of it is highly likely to end up being extracted for domestic use and hence, human consumption. While there is no regulation containing maximum activity concentration or radionuclide guidance values for water that may be destined for uses other than public consumption, if groundwater is considered a “part” of the land, dose criteria for site release can be applied. Therefore, together with the guidance levels to be established for the different radionuclides expected in the groundwater, the detection limits to be employed when performing routine radio analytical characterization procedures in the laboratory should also be provided. In this paper, we first propose a relation of the potential radionuclides to be analyzed in groundwater, together with their detection limits to be achieved when the determinations are performed in a laboratory, and subsequently, we discuss the most suitable analytical methodologies and resources that would be necessary to undertake radiological characterization plans from a practical point of view. |
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2405-8440 |
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THL @ christoph.kuells @ petisco-ferrero_radiological_2023 |
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133 |
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Robin, V.; Beaufort, D.; Tertre, E.; Reinholdt, M.; Fromaget, M.; Forestier, S.; Boissezon, H. de; Descostes, M. |
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Fate of dioctahedral smectites in uranium roll front deposits exploited by acidic In Situ Recovery (ISR) solutions |
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Journal Article |
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Year |
2020 |
Publication |
Applied Clay Science |
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187 |
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105484 |
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Dissolution, In situ recovery, Ion exchange, Post mining, Remediation, Smectite |
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In Situ Recovery (ISR) is the most important process of uranium production in the world (50%). It consists of an injection of a leaching solution into a permeable mineralized aquifer (sandstone), pumping of the solution after dissolution of the ore minerals and recovery of the uranium from the pregnant solution in a surface plant. In this context, the fate of swelling clay minerals such as smectites is of main importance due to their role in the mobility of cationic elements by diverse geochemical processes such as ion-exchange reactions or dissolution. The present study details analysis of dioctahedral smectites before and after in-situ leaching by acidic (H2SO4) ISR solutions. Samples were collected from two sedimentary basins hosting some of the main uranium roll front deposits exploited by acidic ISR (Tortkuduk deposit, Shu-Saryssu basin, Kazakhstan, and Dulaan Uul and Zoovch Ovoo deposits, Sainshand basin, Mongolia). Scanning Electron Microscope and X-Ray Diffraction analysis revealed that dioctahedral smectite is a ubiquitous mineral in all analyzed samples, before and after acidification, and revealed a difference of crystal chemistry of the smectites between deposits of Kazakhstan (beidellite type) and Mongolia (montmorillonite type). Chemical analysis and semi-quantification of the smectites before and after acidification also revealed a difference in chemical reactivity, with a higher dissolution of montmorillonite layers compared to beidellite ones, and the importance of ion-exchange reactions. These findings are consistent with literature data obtained on model systems. The persistence of dioctahedral smectites after several years of acidification is crucial for the understanding of geochemical processes during uranium production or remediation of the aquifers. Finally, based on the analysis of samples from U-deposits hosted in both sedimentary basins, a schematic model of the impact of acid solutions on dioctahedral smectite was proposed. |
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0169-1317 |
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THL @ christoph.kuells @ robin_fate_2020 |
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179 |
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Tanwer, N.; Arora, V.; Kant, K.; Singh, B.; Laura, J.S.; Khosla, B. |
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Chapter 17 – Prevalence of Uranium in groundwater of rural and urban regions of India |
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Book Chapter |
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2024 |
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Water Resources Management for Rural Development |
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213-234 |
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Distribution, Heath impacts, Remediation techniques, Sources, Uranium |
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Abnormally high uranium (U) prevalence in groundwater is a neoteric subject of concern throughout the world because of its direct impact on human health and well-being. Groundwater is used as the most preferred choice for drinking because of its good quality and ease of availability in rural and urban parts of India, and also in different parts of the world. India is an agriculture-dominant country and its 50–80% irrigational requirement is met by groundwater, besides this nearly 90% of rural and 50% of urban water needs are fulfilled by groundwater. The uranium concentration in groundwater in different parts of India namely Punjab, Haryana, Rajasthan, Madhya Pradesh, Karnataka, etc. found to be varying from 0 mg/L to 1443 mg/L, and in different parts of the world, it is found up to 1400 mg/L in the countries like United States, Canada, Finland, Mongolia, Nigeria, South Korea, Pakistan, Burundi, China, Afghanistan, etc. Various natural factors such as geology, hydro-geochemistry, and prevailing conditions as well as anthropogenic factors including mining, nuclear activities, erratic use of fertilizers, and overexploitation of groundwater resources are responsible for adding uranium in groundwater. Groundwater is considered a primary source of uranium ingestion in human beings as it contributes 85% while food contributes 15%. Uranium affects living beings as a two-way sword, being a radioactive element, causing radiotoxicity, and on the other hand as a heavy metal, it causes chemotoxicity. The main target organs affected by the consumption of uranium-contaminated water are kidneys, bones, lungs, etc. It can cause renal failure, impair cell functioning and bone growth, and mutation in DNA. Although, its toxic effects, being a heavy metal, are more severe than its radiotoxicity. Various techniques are available for the efficient removal of uranium from the groundwater such as bioremediation, nanotechnology-enhanced remediation, adsorption, filtration, etc. This chapter entails a comprehensive investigation of uranium contamination in groundwater of rural and urban parts of India their probable sources, health impacts, treatment, and mitigation techniques available to manage groundwater resources. |
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Elsevier |
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Madhav, S.; Srivastav, A.L.; Izah, S.C.; Hullebusch, E. van |
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978-0-443-18778-0 |
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THL @ christoph.kuells @ madhav_chapter_2024 |
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152 |
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Zhang, H.; Gao, J.; Xu, L.; Zhang, X. |
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Case studies of radioactivity of drilling mud for in situ leaching uranium mining in China |
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Journal Article |
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2022 |
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Journal of Environmental Radioactivity |
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251-252 |
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106982 |
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Drilling mud, Exemption management, In situ leaching, Radioactivity |
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The drilling mud from in situ leaching uranium mining is a type of low-radioactivity waste that contains natural nuclides and other harmful substances. In order to determine whether the drilling mud can meet the requirements of radioactive exemption management standards, field investigations and data simulations were conducted in this study. Two typical uranium mines were selected for onsite investigations. Drilling mud from different layers (i.e., the upper covering layer and ore-bearing layer) and from different stages (e.g., logging stage mud, drilling expansion stage mud, and mixed mud) was sampled. For each sample, the 238U and 226Ra concentrations of the solid components and the U and 226Ra concentrations of the supernatant were analyzed. The results revealed that the highest 238U and 226Ra concentrations of the solid components were 4122 Bq/kg and 4077 Bq/kg, while the 238U and 226Ra concentrations of the mixed drilling mud were all less than 300 Bq/kg. A radioactivity estimation model was established for scenario analysis. Exemption management screening lines of waste drilling mud, which can be used to classify and treat the drilling project according to the deposit’s grade and conditions, were proposed for in situ leaching drilling projects. |
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0265-931x |
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THL @ christoph.kuells @ zhang_case_2022 |
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191 |
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Borrego-Alonso, D.; Quintana-Arnés, B.; Lozano, J.C. |
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Natural radionuclides behaviour in drinking groundwaters from Castilla y León (Spain); radiological implications |
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Journal Article |
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2023 |
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Water Research |
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245 |
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120616 |
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Drinking water, Environmental monitoring, Natural radioactivity, Public health, Radiological characterisation |
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Since the coming into force of the European Council Directive 51/2013 EURATOM and its transposition into the Spanish legislation, the presence of radioactive substances in drinking waters must be kept under surveillance to ensure that the health protection requirements are met. Driven by this regulatory framework, in an attempt to know the starting point from which to design surveillance plans, the groundwaters intended for human consumption of Castilla y León (Spain) have been radiologically characterised by using both low-level γ-ray and α-particle spectrometry to determine the activity concentration of the natural radionuclides needed to account for the indicative dose estimation. This extensive research has comprised the radiological characterisation of more than 400 drinking water samples from one of the European Union’s largest regions. Furthermore, the gross α and gross β activities have been analysed. Results showed a high geographical variability that can be related to the hydrogeological formations where the groundwaters come from. The uranium isotopes, 234U and 238U, are the main radionuclides present in the analysed drinking waters reaching values up to 2000 mBq/L, in the southwestern and western of Castilla y León, where U-rich minerals are part of the host rock. High 210Pb and 226,228Ra occurrences are found in the low permeability igneous and metasedimentary hydrogeological formations of Salamanca province. From a public health protection point of view, 4.4% of the total drinking water samples from intakes exceeded the Indicative Dose parametric value of 0.1 mSv, which is a not negligible number of samples, being very likely related to granitic and metamorphosed host rock under specific local conditions. This fact highlights the need for research and consideration of special surveillance of the groundwaters from these areas. |
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0043-1354 |
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THL @ christoph.kuells @ borrego-alonso_natural_2023 |
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157 |
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Liesch, T.; Hinrichsen, S.; Goldscheider, N. |
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Uranium in groundwater — Fertilizers versus geogenic sources |
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Journal Article |
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2015 |
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Science of The Total Environment |
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536 |
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981-995 |
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Keywords |
Drinking water, Fertilizer, Geogenic background, Groundwater, Uranium |
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Abstract |
Due to its radiological and toxicological properties even at low concentration levels, uranium is increasingly recognized as relevant contaminant in drinking water from aquifers. Uranium originates from different sources, including natural or geogenic, mining and industrial activities, and fertilizers in agriculture. The goal of this study was to obtain insights into the origin of uranium in groundwater while differentiating between geogenic sources and fertilizers. A literature review concerning the sources and geochemical processes affecting the occurrence and distribution of uranium in the lithosphere, pedosphere and hydrosphere provided the background for the evaluation of data on uranium in groundwater at regional scale. The state of Baden-Württemberg, Germany, was selected for this study, because of its hydrogeological and land-use diversity, and for reasons of data availability. Uranium and other parameters from N=1935 groundwater monitoring sites were analyzed statistically and geospatially. Results show that (i) 1.6% of all water samples exceed the German legal limit for drinking water (10μg/L); (ii) The range and spatial distribution of uranium and occasional peak values seem to be related to geogenic sources; (iii) There is a clear relation between agricultural land-use and low-level uranium concentrations, indicating that fertilizers generate a measurable but low background of uranium in groundwater. |
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0048-9697 |
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no |
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THL @ christoph.kuells @ liesch_uranium_2015 |
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145 |
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