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Wilson, G.B.; McNeill, G.W. |
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Title |
Noble gas recharge temperatures and the excess air component |
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Journal Article |
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Year |
1997 |
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Applied Geochemistry |
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12 |
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6 |
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747-762 |
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The calculation of a groundwater recharge temperature based on the dissolved concentrations of Ne, Ar, Kr and Xe requires a correction for noble gas supersaturation due to excess air entrainment. This entrainment is commonly attributed to the recharge process or to air contamination at the wellhead during sample collection. With the exception of some local studies, most work has concentrated on interpretation of the recharge temperature or quantification of the radiogenic content for palaeoclimatic and dating purposes. The magnitude and source of the excess air is not directly relevant to these studies and so is often ignored. In this work, excess air Ne and other data have been calculated from new and published noble gas data sets for several groundwater systems. For younger groundwaters which have been recharged under one broad climatic regime, the amount of air entrainment increases according to lithology in the order granites, sandstones and limestones respectively. A negative correlation between precipitation and excess air entrainment is identified in at least one aquifer, and some of the mechanisms which may influence the entrainment process are discussed. |
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THL @ christoph.kuells @ Wilson1997747 |
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281 |
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Vogel, J.C.; Talma, A.S.; Heaton, T.H.E.; Kronfeld, J. |
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Title |
Evaluating the rate of migration of an uranium deposition front within the Uitenhage Aquifer |
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Journal Article |
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Year |
1999 |
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Journal of Geochemical Exploration |
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66 |
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1 |
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269-276 |
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redox changes in aquifer, sandstone-type uranium deposit, South Africa, uranium series |
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The solubility of uranium in groundwater is very sensitive to changes in redox conditions. Many secondary (sandstone-type) uranium deposits have been formed when soluble U has precipitated after encountering reducing conditions in the subsurface. In the groundwater of the Uitenhage Aquifer (Cape Province, South Africa), 238U-series isotopes were used to assist in studying the history of the reducing barrier. Uranium isotopes were used to determine the present position of the barrier. Radium and radon were used to evaluate the path of migration that the front of the oxygen depletion zone has taken over the past 105 years. During this time the reducing barrier has moved, leaving in its wake a trail of U in various stages of secular equilibrium with its daughter 230Th. The 226Ra daughter of 230Th is not very mobile. Its growth upon the aquifer wall is reflected in the Rn content of the water. This in turn, due to the relatively great age of the water, indicates the extent of the 230Th ingrowth (from precipitated U) that took place before the barrier migrated. |
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0375-6742 |
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THL @ christoph.kuells @ vogel_evaluating_1999 |
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126 |
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Hubbard, B.E.; Gallegos, T.J.; Stengel, V.; Hoefen, T.M.; Kokaly, R.F.; Elliott, B. |
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Title |
Hyperspectral (VNIR-SWIR) analysis of roll front uranium host rocks and industrial minerals from Karnes and Live Oak Counties, Texas Coastal Plain |
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Journal Article |
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Year |
2024 |
Publication |
Journal of Geochemical Exploration |
Abbreviated Journal |
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Volume |
257 |
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107370 |
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Critical minerals, Hyperspectral, Industrial minerals, Mine waste, Texas coastal plain, Uranium |
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VNIR-SWIR (400–2500 nm) reflectance measurements were made on the surfaces of various cores, cuttings and sample splits of sedimentary rocks from the Tertiary Jackson Group, and Catahoula, Oakville and Goliad Formations. These rocks vary in composition and texture from mudstone and claystone to sandstone and are known host rocks for roll front uranium occurrences in Karnes and Live Oak Counties, Texas. Spectral reflectance profiles, 569 in total, were reduced to 125 representative spectral signatures, which were analyzed using the U.S. Geological Survey’s (USGS) Material Identification and Characterization Algorithm (MICA). MICA uses an automated continuum-removal procedure together with a least-squares linear regression to determine the fit of observed sample spectral absorption features to those of reference mineral standards in a spectral library. The reference minerals include various clay, mica, carbonate, ferric and ferrous iron minerals and their mixtures. In addition, absorption feature band-depth analysis was done to identify rock surfaces exhibiting absorption features related to uranium and zeolite minerals, which were not included in the command files used to execute MICA. Rocks from each of the four geologic units produced broadly similar spectral signatures as a result of comparable mineral compositions, but there were some notable differences. For example, Ca- and Na-montmorillonite was matched most frequently to the spectral absorption features in 2-μm (∼2000–2500 nm) wavelengths, while goethite occurred often at 1-μm (∼400–1000 nm) wavelengths. The latter is related to limonitic iron-staining in and around oxidized zones of the uranium roll front as described in previous papers. Rocks of the Jackson Group differed from those of the Catahoula, Oakville and Goliad units in that the former exhibited spectral features we interpret as being due to the presence of lignite-bearing mudstone layers. Goliad rocks exhibit spectral features related to dolomite, gypsum, anhydrite, and an unidentified green clay mineral that is possibly glauconite. Jackson Group rocks also exhibit weak but well-resolved absorption features at 964 and 1157 nm related to either or both zeolite minerals clinoptilolite and heulandite. These zeolite minerals and a few spectra exhibiting hydrous silica absorption features are indicative of alteration of volcanic glass in tuffaceous mudstone and claystone layers. A few sample spectra exhibited strong absorption features at around 1135 nm related to the uranium mineral coffinite. Both the 1135 nm coffinite and 1157 nm zeolite absorption features overlap somewhat, potentially making them difficult to distinguish without additional hyperspectral field, laboratory or remote sensing data. The results of this study were compared to mixtures of minerals described for ore, gangue and alteration minerals in deposit models for sandstone-hosted uranium, sedimentary bentonite and sedimentary zeolite. Use of these spectra can help facilitate mapping of both waste materials from the legacy mining of the above commodities, as well as future exploration and resource assessment activities. |
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THL @ christoph.kuells @ hubbard_hyperspectral_2024 |
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178 |
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Grozeva, N.G.; Radwan, J.; Beaucaire, C.; Descostes, M. |
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Title |
Reactive transport modeling of U and Ra mobility in roll-front uranium deposits: Parameters influencing 226Ra/238U disequilibria |
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Journal Article |
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Year |
2022 |
Publication |
Journal of Geochemical Exploration |
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236 |
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106961 |
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Keywords |
Ra/U, Radioactive disequilibria, Radium, Reactive transport modeling, Roll-front uranium deposit |
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Abstract |
Uranium reserve estimates in ore deposits can be significantly impacted by 226Ra/238U disequilibria arising from the differential mobility of uranium and radium during groundwater transport. 1D reactive transport models were developed to investigate the long-term effects of retention processes (UO2(am) precipitation, U(VI) and Ra sorption on smectite, Ra co-precipitation with barite) on the repartitioning of 238U and 226Ra during formation of roll-front type deposits. Analytical solutions to radioactive decay chains were used in complement to examine the influence of geochemical parameters, including fluid 234U/238U activity ratios and α-recoil loss, on 226Ra/238U disequilibria in uranium ores. Model results demonstrate that smectite and barite can produce 226Ra/238U ratios \textgreater1 at low uranium contents and may explain 226Ra/238U disequilibria occurring in altered rock up- and downstream of roll-front deposits. The capacity of these phases to take up Ra and generate 226Ra/238U disequilibria depends on both mineral contents and groundwater compositions, and is thus expected to be site-specific. Simulations of ore deposits that advance downstream with time demonstrate the formation of stronger 226Ra/238U disequilibria, as expected, in the downgradient side or nose of the ore, reflecting both younger mineralization ages and the presence of active uranium precipitation. Whether disequilibria are positive or negative with respect to secular equilibrium, however, depends on the 234U/238U activity ratio in the fluid from which uranium minerals precipitate. Smaller hydraulic conductivities are shown to generate a narrower range in 226Ra/238U activity ratios with distance, and may explain the occurrence of disequilibria in the limb ore that are less pronounced than those in the nose. Furthermore, the ability of α-recoil loss to decrease 226Ra/238U activity ratios at secular equilibrium may account for negative disequilibria in high grade ores. The South Tortkuduk uranium deposits (Kazakhstan) are subsequently used as a case study to identify the processes and parameters that may contribute to 226Ra/238U disequilibria at this site. Variations in multiple parameters, including clay contents, barite contents, and mineralization ages, are found to reproduce measured 226Ra/238U activity ratios in the roll-front ore. Prioritization of these parameters will necessitate field measurements targeting both groundwater fluids and the host rock. Results from this study will ultimately aid geologists in building appropriate hydrogeochemical data sets to more efficiently locate and exploit uranium ore deposits. |
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0375-6742 |
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THL @ christoph.kuells @ grozeva_reactive_2022 |
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180 |
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Author |
Boulesteix, T.; Cathelineau, M.; Deloule, E.; Brouand, M.; Toubon, H.; Lach, P.; Fiet, N. |
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Title |
Ilmenites and their alteration products, sinkholes for uranium and radium in roll-front deposits after the example of South Tortkuduk (Kazakhstan) |
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Journal Article |
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Year |
2019 |
Publication |
Journal of Geochemical Exploration |
Abbreviated Journal |
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206 |
Issue |
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Pages |
106343 |
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Abstract |
The approximate determination of average Ra/U disequilibria in orebodies is one of the most common causes of errors in U reserve estimations. In roll-front deposits, the disequilibria are however frequently distributed following complex geometries, which must be fully understood to prevent major U reserve overestimates and costly unproductive extractive operations. The processes responsible for disruption of the radioactive equilibria and the U and Ra carriers in such complex natural systems remain poorly constrained. In this contribution, we propose an innovative approach, mixing orebody to sub-grain scale studies to unravel the distribution of U and Ra and the processes responsible for their concentration and uncoupling. Using mineral separations, gamma spectrometry and mineral-chemical analyses, we identified the Fe-Ti clusters (altered ilmenite + pyrite/marcasite) as the microsites for coffinite precipitation and Ra concentration. To understand the influence of such clusters on the distribution of U and Ra at the deposit scale, whole-rock Ra/U disequilibria were measured and mapped at a series of ten drill holes along a profile crosscutting the studied roll-front. The main Ra/U disequilibria are encountered around the mineralization in low U content zones. They are controlled by two main processes. (1) In the oxidized zones, the immobility of 230Th with respect to the U produces patches of Ra disequilibria (carried by the altered U minerals). (2) In the immediate vicinity of the roll-front, the dissolution of the mineralization produces an Ra flux trapped by the alteration products of ilmenites, as definitely confirmed by direct SIMS measurements. Such a process is responsible for the Ra disequilibria envelope located downstream of the richest ores, also known as Ra halo. The highest Ra/U ratios correspond to oxidized upstream samples, but most other high Ra/U ratios are from reduced downstream samples close to the mineralization. Such a low to medium U content envelope with high Ra/U ratios constitutes the main cause of U reserve overestimations. |
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0375-6742 |
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THL @ christoph.kuells @ boulesteix_ilmenites_2019 |
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181 |
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Hebert, B.; Baron, F.; Robin, V.; Lelievre, K.; Dacheux, N.; Szenknect, S.; Mesbah, A.; Pouradier, A.; Jikibayev, R.; Roy, R.; Beaufort, D. |
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Quantification of coffinite (USiO4) in roll-front uranium deposits using visible to near infrared (Vis-NIR) portable field spectroscopy |
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Journal Article |
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Year |
2019 |
Publication |
Journal of Geochemical Exploration |
Abbreviated Journal |
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199 |
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53-59 |
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Coffinite, Mineral quantification, Near infrared, Ore exploration, Portable field spectroscopy, Roll-front deposits |
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Coffinite (USiO4) is a common uranium-bearing mineral of roll-front uranium deposits. This mineral can be identified by the visible near infrared (Vis-NIR) portable field spectrometers used in mining exploration. However, due to the low detection limits and associated errors, the quantification of coffinite abundance in the mineralized sandstones or sandy sediments of roll-front uranium deposits using Vis-NIR spectrometry requires a specific methodological development. In this study, the 1135 nm absorption band area is used to quantify the abundance of coffinite. This absorption feature does not interfere with NIR absorption bands of any other minerals present in natural sands or sandstones of uranium roll-front deposits. The correlation between the 1135 nm band area and coffinite content was determined from a series of spectra measured from prepared mineral mixtures. The samples were prepared with a range of weighted amounts of arenitic sands and synthetic coffinite simulating the range of uranium concentration encountered in roll-front uranium deposits. The methodology presented in this study provides the quantification of the coffinite content present in sands between 0.03 wt% to 1 wt% coffinite with a detection limit as low as 0.005 wt%. The integrated area of the 1135 nm band is positively correlated with the coffinite content of the sand in this range, showing that the method is efficient to quantify coffinite concentrations typical of roll-front uranium deposits. The regression equation defined in this study was then used as a reference to predict the amount of natural coffinite in a set of mineralized samples from the Tortkuduk uranium roll-front deposit (South Kazakhstan). |
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0375-6742 |
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THL @ christoph.kuells @ hebert_quantification_2019 |
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184 |
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Bullock, L.A.; Parnell, J. |
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Selenium and molybdenum enrichment in uranium roll-front deposits of Wyoming and Colorado, USA |
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Journal Article |
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Year |
2017 |
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Journal of Geochemical Exploration |
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180 |
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101-112 |
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Molybdenum, Roll-fronts, Selenium, Tellurium, Uranium, Wyoming |
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Sandstone uranium (U) roll-front deposits of Wyoming and Colorado (USA) are important U resources, and may provide a terrestrial source for critical accessory elements, such as selenium (Se), molybdenum (Mo), and tellurium (Te). Due to their associated toxicity, MoSeTe occurrences in roll-fronts should also be carefully monitored during U leaching and ore processing. While elevated MoSe concentrations in roll-fronts are well established, very little is known about Te occurrence in such deposits. This study aims to establish MoSeTe concentrations in Wyoming and Colorado roll-fronts, and assess the significance of these deposits in an environmental and mineral exploration context. Sampled roll-front deposits, produced by oxidized groundwater transportation through a sandstone, show high MoSe content in specific redox zones, and low Te, relative to crustal means. High Se concentrations (up to 168ppm) are restricted to a narrow band of alteration at the redox front. High Mo content (up to 115ppm) is typically associated with the reduced mineralized nose and seepage zones of the roll-front, ahead of the U orebody. Elevated trace element concentrations are likely sourced from proximal granitic intrusions, tuffaceous deposits, and local pyritic mudstones. Elevated MoSe content in the sampled roll fronts may be regarded as a contaminant in U in-situ recovery and leaching processing, and may pose an environmental threat in groundwaters and soils, so extraction should be carefully monitored. The identification of peak concentrations of MoSe can also act as a pathfinder for the redox front of a roll-front, and help to isolate the U orebody, particularly in the absence of gamma signatures. |
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0375-6742 |
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THL @ christoph.kuells @ bullock_selenium_2017 |
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189 |
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Stavi, I.; Eldad, S.; Xu, C.; Xu, Z.; Gusarov, Y.; Haiman, M.; Argaman, E. |
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Ancient agricultural terrace walls control floods and regulate the distribution of Asphodelus ramosus geophytes in the Israeli arid Negev |
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Journal Article |
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2024 |
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Catena |
Abbreviated Journal |
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234 |
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107588 |
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Geo-archaeology, Hydrological connectivity, Hydrological modelling, Runoff harvesting, Soil and water conservation, Watershed management |
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Ancient stone terrace walls aimed at harvesting water runoff and facilitating crop production are widespread across the drylands of the Middle East and beyond. In addition to retaining the scarce water resource, the terrace walls also conserve soil and thicken its profile along ephemeral stream channels (wadis) by decreasing fluvial connectivity and mitigating erosional processes. In this study, we created hydrological models for three wadis with ancient stone terrace walls in the arid northern Negev of Israel, where the predominant geophyte species is Asphodelus ramosus L. A two-dimensional (2D) rain-on-grid (RoG) approach with a resolution of 2 m was used to simulate the rain events with return periods of 10, 20, 50, and 99 % (10-y, 5-y, 2-y, and yearly, respectively) based on the Intensity-Duration-Frequency rain curves for the region. To evaluate the effect of stone terrace walls on fluvial hydrology and geomorphology, the ground level was artificially elevated by 20 cm at the wall locations in a digital terrain model (DTM), using the built-in HEC-RAS 2D terrain modification tool. Our results showed that the terraced wadis have a high capacity to mitigate runoff loss, but a lesser capacity to delay the peak flow. Yet, for all rainstorm return periods, peak flow mitigation was positively related to the number of terrace walls along the stream channel. Field surveys in two of the studied wadis demonstrated that the A. ramosus clones were found in proximity to the stone terrace walls, presumably due to the greater soil–water content there. The results thus suggest that the terrace walls provide improved habitat conditions for these geophytes, supporting their growth and regulating their distribution along the wadi beds. |
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0341-8162 |
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THL @ christoph.kuells @ Stavi2024107588 |
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229 |
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Jing, M.; Kumar, R.; Attinger, S.; Li, Q.; Lu, C.; Heße, F. |
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Assessing the contribution of groundwater to catchment travel time distributions through integrating conceptual flux tracking with explicit Lagrangian particle tracking |
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Journal Article |
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2021 |
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Advances in Water Resources |
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149 |
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103849 |
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Travel time distribution, Flux tracking, Particle tracking, Coupled model, Predictive uncertainty |
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Travel time distributions (TTDs) provide an effective way to describe the transport and mixing processes of water parcels in a subsurface hydrological system. A major challenge in characterizing catchment TTD is quantifying the travel times in deep groundwater and its contribution to the streamflow TTD. Here, we develop and test a novel modeling framework for an integrated assessment of catchment scale TTDs through explicit representation of 3D-groundwater dynamics. The proposed framework is based on the linkage between a flux tracking scheme with the surface hydrologic model (mHM) for the soil-water compartment and a particle tracking scheme with the 3D-groundwater model OpenGeoSys (OGS) for the groundwater compartment. This linkage provides us with the ability to simulate the spatial and temporal dynamics of TTDs in these different hydrological compartments from grid scale to regional scale. We apply this framework in the Nägelstedt catchment in central Germany. Simulation results reveal that both shape and scale of grid-scale groundwater TTDs are spatially heterogeneous, which are strongly dependent on the topography and aquifer structure. The component-wise analysis of catchment TTD shows a time-dependent sensitivity of transport processes in soil zone and groundwater to driving meteorological forcing. Catchment TTD exhibits a power-law shape and fractal behavior. The predictive uncertainty in catchment mean travel time is dominated by the uncertainty in the deep groundwater rather than that in the soil zone. Catchment mean travel time is severely biased by a marginal error in groundwater characterization. Accordingly, we recommend to use multiple summary statistics to minimize the predictive uncertainty introduced by the tailing behavior of catchment TTD. |
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0309-1708 |
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THL @ christoph.kuells @ Jing2021103849 |
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220 |
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Timsina, J.; Weerahewa, J. |
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Title |
Restoring ancient irrigation systems for sustainable agro-ecosystems development: Reflections on the special issue |
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Journal Article |
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2023 |
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Agricultural Systems |
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209 |
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103668 |
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Keywords |
Ancient irrigation systems, Degradation, Sustainability, Sri Lanka |
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Abstract |
Humans have relied on agriculture to feed their communities for thousands of years. Irrigation is practiced in many different forms over the years in countries all over the world. Although modern irrigation systems have been developed, and are in use in many countries, ancient irrigation systems (AISs) have also played a major role in sustaining food production, especially in smallholder farming in least developed and developing countries. The editorial team of Agricultural Systems put out a call for a special issue on restoring AISs for sustainable agro-ecosystems development to capture ancient marvels of traditional irrigation technology across the world. The objectives of this special issue were to: (i) understand and analyse the hydrological and socio-economic networks anchored by AISs; (ii) explain the nature and sustainability of management of these systems in relation to local agro-ecosystems; (iii) analyse the implications of the AISs for land, soil and water quality, and agro-ecosystem services; (iv) qualitative and quantitative analysis of AISs, including bio-physical and bio-economic modelling of these systems; and (v) assess the feasibility of alternative technological, institutional and management strategies to enhance the productivity, profitability, and environmental sustainability of the systems. The overall goal of the special issue was to develop a useful repository for this information as well as to use the journal’s international reach to share this information with the agricultural systems research community and journal readership. This paper provides reflections of papers published in the special issue. The special issue resulted in twelve high quality original research articles and one review article from Asia, Africa and Europe. The findings from various papers revealed that the AISs have been degraded due to human interventions or the anthropogenic activities across the world. Various papers emphasized that as a corrective measure, there is a need for developing and implementing rehabilitation projects in these systems. Authors identified that appropriate policy interventions by the relevant authorities would be a major step towards such rehabilitation process. However, resetting the ecosystem structure of the AISs strictly towards their historical manifestation is neither required nor feasible in the present context as it would contradict the expectations of stakeholders from these systems. The knowledge generated through the special issue provides evidence-based information on various aspects of AISs. It helps aware governments, private sectors and development agencies for improved policy planning and decision making and for prioritizing the restoration, rehabilitation, and management of various AISs around the world. |
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0308-521x |
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THL @ christoph.kuells @ Timsina2023103668 |
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255 |
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