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Paradis, C.J.; Hoss, K.N.; Meurer, C.E.; Hatami, J.L.; Dangelmayr, M.A.; Tigar, A.D.; Johnson, R.H. |
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Elucidating mobilization mechanisms of uranium during recharge of river water to contaminated groundwater |
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Journal Article |
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2022 |
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Journal of Contaminant Hydrology |
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251 |
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104076 |
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Desorption, Dissolution, Groundwater, Surface water, Tracer, Uranium |
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The recharge of stream water below the baseflow water table can mobilize groundwater contaminants, particularly redox-sensitive and sorptive metals such as uranium. However, in-situ tracer experiments that simulate the recharge of stream water to uranium-contaminated groundwater are lacking, thus limiting the understanding of the potential mechanisms that control the mobility of uranium at the field scale. In this study, a field tracer test was conducted by injecting 100 gal (379 l) of oxic river water into a nearby suboxic and uranium-contaminated aquifer. The traced river water was monitored for 18 days in the single injection well and in the twelve surrounding observation wells. Mobilization of uranium from the solid to the aqueous phase was not observed during the tracer test despite its pre-test presence being confirmed on the aquifer sediments from lab-based acid leaching. However, strong evidence of oxidative immobilization of iron and manganese was observed during the tracer test and suggested that immobile uranium was likely in its oxidized state as U(VI) on the aquifer sediments; these observations ruled out oxidation of U(IV) to U(VI) as a potential mobilization mechanism. Therefore, desorption of U(VI) appeared to be the predominant potential mobilization mechanism, yet it was clearly not solely dependent on concentration as evident when considering that uranium-poor river water (\textless0.015 mg/L) was recharged to uranium-rich groundwater (≈1 mg/L). It was possible that uranium desorption was limited by the relatively higher pH and lower alkalinity of the river water as compared to the groundwater; both factors favor immobilization. However, it was likely that the immobile uranium was associated with a mineral phase, as opposed to a sorbed phase, thus desorption may not have been possible. The results of this field tracer study successfully ruled out two common mobilization mechanisms of uranium: (1) oxidative dissolution and (2) concentration-dependent desorption and ruled in the importance of advection, dispersion, and the mineral phase of uranium. |
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0169-7722 |
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THL @ christoph.kuells @ paradis_elucidating_2022 |
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135 |
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Ren, Y.; Yang, X.; Hu, X.; Wei, J.; Tang, C. |
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Title |
Mineralogical and geochemical evidence for biogenic uranium mineralization in northern Songliao Basin, NE China |
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Journal Article |
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Year |
2022 |
Publication |
Ore Geology Reviews |
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141 |
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104556 |
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Bacterial sulfate reduction, In-situ S isotope of pyrite, Northern Songliao basin, Sandstone-type uranium deposit, Sifangtai Formation |
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The sandstone-hosted uranium mineralization areas in the Sanzhao Sag of the northern Songliao Basin have been newly identified. The target stratum is the Upper Cretaceous Sifangtai Formation and the uranium mineralization mainly occurs in the bottom of Sifangtai Formation, corresponding to channel sand bodies in meandering river system, characterized by medium to fine-grained sandstone. This study proposes the uranium metallogenic model through petrographic observation, whole rock geochemistry, mineralogical study of uranium occurrence form (SEM), organic matter rock–eval pyrolysis analysis (REP) and in-situ sulfur isotope determination of different generations of pyrite by LA-MC-ICP-MS. Compared with the sandstones collected in barren reduction and oxidization zones, the mineralized sandstones show obvious increase in the contents of TOC, total sulfur, Y and U. Petrographic observations indicate that organic matters are mainly inherited from land plants. REP data display that the organic matter (OM) disseminated in the sandstone has very low hydrogen index (HI) from around 0 to 21 mg HC/g TOC and varied oxygen index (OI) from 44 to 115 mg CO2/g TOC, corresponding to Type Ⅳ kerogen (degraded kerogen). There are two types of coffinite with different grain size, micro-particles (μm-sized) and large aggregates (generally up to 100 μm) respectively. The coffinite micro spherules exhibit short rod-like or worm-like morphology occurring in clay matrix and cell cavities in degradofusinite or around subidiomorphic-idiomorphic pyrite. The coarse-grained coffinite contains other mineral facies (e.g. pyrite, quartz) and some of large coffinite aggregates display thrombolite-type microbial structures. The irregular pyrite relict particles in coarse-grained colloidal coffinite have light sulfur isotope compositions characterized by δ34S values from –39.96‰ to –49.89‰. The δ34S values of colloidal pyrite in replacement of OM or of the sub-idiomorphic FeS2 cement filling in the cavities of OM range from –52.77‰ to –13.88‰. Some of sub-idiomorphic pyrite cement and idiomorphic crystal have the heavier signature from – 27.06‰ to + 14.23‰. The light sulfur isotope signature suggests that the sulfur originates from bacterial sulfate reduction (BSR). The OM replacement by pyrite and the highest OI values recorded by REP in uranium mineralized samples are lines of evidence of biodegradation. Bacteria use the organic matter as food source and produce isotopically light reduced sulfur species. Oxygenated uranium-bearing waters infiltrated through the denudated windows at Daqing placanticline into the porous reduced sandstones deposited in the Sanzhao Sag. Uranium was indirectly reduced by BSR-derived iron disulfides or directly reduced by sulfate-reducing bacteria. |
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0169-1368 |
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THL @ christoph.kuells @ ren_mineralogical_2022 |
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144 |
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Xiao, L.; Robinson, M.; O’Connor, M. |
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Title |
Woodland’s role in natural flood management: Evidence from catchment studies in Britain and Ireland |
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Journal Article |
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Year |
2022 |
Publication |
Science of The Total Environment |
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813 |
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151877 |
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Forest harvesting, Streamflow, Natural flood management, Before-after-control-impact, Evidence-based forest impact |
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Despite the attention currently given to the potential environmental benefits of large-scale forest planting, there is a shortage of clear observational evidence regarding the effects on river flows, and what there is has often been contradictory or inconclusive. This paper presents three independently conducted paired-catchment forestry studies covering 66 station-years of flow measurements in the UK and Ireland. In each case coniferous evergreen trees were removed from one catchment with minimal soil disturbance while the adjoining control catchment was left unchanged. Trees were removed from 20% – 90% of the three experimental basins. Following woodland removal there was an increase in dry weather baseflow at all sites. Baseflows increased by about 8% after tree removal from a quarter of the Hore basin and by 41% for the near-total cut at Howan. But the changes were more complex for peak flows. Tree harvesting increased the smallest and most frequent peak storm flows, indicating that afforestation would lead to the suppression of such events. This was however restricted to events well below the mean annual flood, indicating that the impact of forests upon the largest and most damaging floods is likely to be limited. Whilst a forest cover can be effective in mitigating small and frequent stormflows it should never be assumed to provide protection against major flood events. |
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0048-9697 |
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THL @ christoph.kuells @ Xiao2022151877 |
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241 |
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Sahoo, P.K.; Virk, H.S.; Powell, M.A.; Kumar, R.; Pattanaik, J.K.; Salomão, G.N.; Mittal, S.; Chouhan, L.; Nandabalan, Y.K.; Tiwari, R.P. |
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Meta-analysis of uranium contamination in groundwater of the alluvial plains of Punjab, northwest India: Status, health risk, and hydrogeochemical processes |
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Journal Article |
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Year |
2022 |
Publication |
Science of The Total Environment |
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807 |
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151753 |
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Agrochemicals, Geogenic contamination, Punjab, Salinity, Shallow aquifer, Uranium enrichment |
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Despite numerous studies, there are many knowledge gaps in our understanding of uranium (U) contamination in the alluvial aquifers of Punjab, India. In this study, a large hydrogeochemical dataset was compiled to better understand the major factors controlling the mobility and enrichment of uranium (U) in this groundwater system. The results showed that shallow groundwaters (\textless60 m) are more contaminated with U than from deeper depths (\textgreater60 m). This effect was predominant in the Southwest districts of the Malwa, facing significant risk due to chemical toxicity of U. Groundwaters are mostly oxidizing and alkaline (median pH: 7.25 to 7.33) in nature. Spearman correlation analysis showed that U concentrations are more closely related to total dissolved solids (TDS), salinity, Na, K, HCO3−, NO3− Cl−, and F− in shallow water than deep water, but TDS and salinity remained highly correlated (U-TDS: ρ = 0.5 to 0.6; U-salinity: ρ = 0.5). This correlation suggests that the salt effect due to high competition between ions is the principal cause of U mobilization. This effect is evident when the U level increased with increasing mixed water species (Na-Cl, Mg-Cl, and Na-HCO3). Speciation data showed that the most dominant U species are Ca2UO2(CO3)2− and CaUO2(CO3)3−, which are responsible for the U mobility. Based on the field parameters, TDS along with pH and oxidation-reduction potential (ORP) were better fitted to U concentration above the WHO guideline value (30 μg.L−1), thus this combination could be used as a quick indicator of U contamination. The strong positive correlation of U with F− (ρ = 0.5) in shallow waters indicates that their primary source is geogenic, while anthropogenic factors such as canal irrigation, groundwater table decline, and use of agrochemicals (mainly nitrate fertilizers) as well as climate-related factors i.e., high evaporation under arid/semi-arid climatic conditions, which result in higher redox and TDS/salinity levels, may greatly affect enrichment of U. The geochemical rationale of this study will provide Science-based-policy implications for U health risk assessment in this region and further extrapolate these findings to other arid/semi-arid areas worldwide. |
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0048-9697 |
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THL @ christoph.kuells @ sahoo_meta-analysis_2022 |
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150 |
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Kazemi, A.; Esmaeilbeigi, M.; Sahebi, Z.; Ansari, A. |
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Health risk assessment of total chromium in the qanat as historical drinking water supplying system |
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Journal Article |
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2022 |
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Science of The Total Environment |
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807 |
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150795 |
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Qanat, Total chromium, Hazard quotient, Non-carcinogenic risk, Risk assessment, Eastern Iran |
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This study investigated the health risk assessment of total chromium (CrT) in qanats of South Khorasan, Eastern Iran. For this, concentration of CrT in a total of 83 qanats were measured in summer 2020. Samples were initially tested in the field for temperature, pH, dissolved oxygen (DO), electrical conductivity (EC), and total dissolved solids (TDS). In the lab, collected samples were filtered and fixed with nitric acid (HNO3) for the detection of CrT using inductively coupled plasma mass spectrometry (ICP-MS). Hazard quotient (HQ) and carcinogenic risk assessments were considered to evaluate the risks of CrT to inhabitants. Results showed that concentration of CrT ranged from 1.79 to 1017.05 μg L-1, and a total of 25 stations illuminated CrT concentrations above the WHO standards (50 μg L-1). HQ demonstrated HQ < 1 for 90.37% of studied samples with negligible hazard, whereas 9.63% of stations illuminated HQ ≥ 1 meaning the presence of non-carcinogenic risk for water consumers. Carcinogenic risk (CR) exhibited CR > 1.00E-04 in 81.93% of qanats while 18.07% of stations had 1.00E-06 < CR < 1.00E-04 meaning no acceptable and acceptable CR for the studied qanats, respectively. Zoning map displayed that qanats in the south of South Khorasan possessed the highest HQ, but north regions showed the lowest ones. Together, CrT in qanats of South Khorasan is above the WHO limit, which results in a high risk of carcinogenicity for residents, and in turn, more efforts should be made to provide hygienic groundwater for consumers. |
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0048-9697 |
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THL @ christoph.kuells @ Kazemi2022150795 |
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269 |
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Prusty, S.; Somu, P.; Sahoo, J.K.; Panda, D.; Sahoo, S.K.; Sahoo, S.K.; Lee, Y.R.; Jarin, T.; Sundar, L.S.; Rao, K.S. |
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Adsorptive sequestration of noxious uranium (VI) from water resources: A comprehensive review |
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2022 |
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Chemosphere |
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308 |
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136278 |
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Adsorbents, Adsorption, Techniques, Uranium, Wastewater |
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Groundwater is usually utilized as a drinking water asset everywhere. Therefore, groundwater defilement by poisonous radioactive metals such as uranium (VI) is a major concern due to the increase in nuclear power plants as well as their by-products which are released into the watercourses. Waste Uranium (VI) can be regarded as a by-product of the enrichment method used to produce atomic energy, and the hazard associated with this is due to the uranium radioactivity causing toxicity. To manage these confronts, there are so many techniques that have been introduced but among those adsorptions is recognized as a straightforward, successful, and monetary innovation, which has gotten major interest nowadays, despite specific drawbacks regarding operational as well as functional applications. This review summarizes the various adsorbents such as Bio-adsorbent/green materials, metal oxide-based adsorbent, polymer based adsorbent, graphene oxide based adsorbent, and magnetic nanomaterials and discuss their synthesis methods. Furthermore, this paper emphasis on adsorption process by various adsorbents or modified forms under different physicochemical conditions. In addition to this adsorption mechanism of uranium (VI) onto different adsorbent is studied in this article. Finally, from the literature reviewed conclusion have been drawn and also proposed few future research suggestions. |
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0045-6535 |
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THL @ christoph.kuells @ prusty_adsorptive_2022 |
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131 |
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Kumar, V.; Setia, R.; Pandita, S.; Singh, S.; Mitran, T. |
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Assessment of U and As in groundwater of India: A meta-analysis |
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Journal Article |
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2022 |
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Chemosphere |
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303 |
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135199 |
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Arsenic, Geology, Groundwater, Health risk, Soil texture, Uranium |
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More than 2.5 billion people depend upon groundwater worldwide for drinking, and giving quality water has become one of the great apprehensions of human culture. The contamination of Uranium (U) and Arsenic (As) in the groundwater of India is gaining global attention. The current review provides state-of-the-art groundwater contamination with U and As in different zones of India based on geology and soil texture. The average concentration of U in different zones of India was in the order: West Zone (41.07 μg/L) \textgreater North Zone (37.7 μg/L) \textgreater South Zone (13.5 μg/L)\textgreater Central Zone (7.4 μg/L) \textgreater East Zone (5.7 μg/L) \textgreaterSoutheast Zone (2.4 μg/L). The average concentration of As in groundwater of India is in the order: South Zone (369.7 μg/L)\textgreaterCentral Zone (260.4 μg/L)\textgreaterNorth Zone (67.7 μg/L)\textgreaterEast Zone (60.3 μg/L)\textgreaterNorth-east zone (9.78 μg/L)\textgreaterWest zone (4.14 μg/L). The highest concentration of U and As were found in quaternary sediments, but U in clay skeletal and As in loamy skeletal. Results of health risk assessment showed that the average health quotient of U in groundwater for children and adults was less than unity. In contrast, it was greater than unity for As posing a harmful impact on human health. This review provides the baseline data regarding the U and As contamination status in groundwater of India, and appropriate, effective control measures need to be taken to control this problem. |
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0045-6535 |
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THL @ christoph.kuells @ kumar_assessment_2022 |
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161 |
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Wang, B.; Luo, Y.; Liu, J.-hui; Li, X.; Zheng, Z.-hong; Chen, Q.-qian; Li, L.-yao; Wu, H.; Fan, Q.-ren |
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Ion migration in in-situ leaching (ISL) of uranium: Field trial and reactive transport modelling |
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Journal Article |
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2022 |
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Journal of Hydrology |
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615 |
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128634 |
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Acid in situ leaching, Banyan-Uul uranium deposit, Influence area, Reactive transport, Sensitivity analysis |
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Acid in-situ leaching (ISL) can be used as a mining technique for in situ uranium recover from underground. Acids and oxidants as lixiviants were continuously injected into a sandstone-type uranium deposit in Bayan-Uul (China). It was conducted to facilitate the dissolution of uranium minerals to generate uranyl ions, which could then be extracted for the recovery of uranium resources by the pumping cycle. A reactive transport model based on PHAST was developed to investigate the dynamic reactive migration process of uranium. The simulated results well reproduce the fluid dynamic evolution in the injecting and pumping units, as well as the dynamic release of uranium. The simulated leaching area indicates that the uranium ore leaching area was much larger than the acidification area. In addition, the pollution plume of uranium and acid water was larger than that of the leaching area, which can be used as a reference for uranium mining schemes. Furthermore, the parameter sensitivity analysis indicates the volume fraction of uranium ore and the reaction rate were the main factors affecting uranium leaching efficiency. Without considering the blockage of pores by precipitation, the Fe2+ in the reinjection fluid had a significant negative influence on uranium leaching. |
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0022-1694 |
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THL @ christoph.kuells @ wang_ion_2022 |
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195 |
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Rooyen, J.D. van; Watson, A.W.; Miller, J.A. |
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Using tritium and radiocarbon activities to constrain regional modern and fossil groundwater mixing in Southern Africa |
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Journal Article |
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2022 |
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Journal of Hydrology |
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614 |
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128570 |
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Radiocarbon, Residence time, SADC, Tritium |
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This study combines historical records of 14C and 3H in the atmosphere and soil with renewal rate and groundwater lumped parameter models to predict the abundance of 14C and 3H in groundwater over time. 624 groundwater samples from numerous studies, over four decades (1978–2019), in South Africa, Namibia, Botswana and Mozambique were collated to compare with predicted groundwater activities of 14C and 3H within the South African Development Community (SADC) region. Spatial datasets of carbonate bearing lithology, C3/C4 vegetation, summer/winter rainfall and coastal proximity were used to apply corrections to 14C and 3H data. Corrected values of 14C and 3H were compared with the theoretical abundance of these tracers, derived from the lumped parameter models, to estimate the general mean residence times and presence of groundwater mixing between modern recharge and older groundwaters. This study found that corrected values produced varying mean residence times derived from 14C ages (∼500–28500 years) and a wide range of potentially mixed waters within each aquifer system (0–100 % of tested wells) across the study area. The largest proportions of mixed groundwater, as well as the youngest mean residence times, were found in alluvial and primary fractured rock aquifers (e.g., western coast of South Africa and southern Mozambique). The smallest proportions of mixed groundwater were predicted in deep confined clay-rich aquifers as well as layered coal bearing carbonate sequences (e.g., Orapa, Malwewe and Serowe, Botswana). Insights into the proportions of mixed groundwater and mean residence times can help assess hydrological resilience on a regional scale. Such information is pertinent in promoting socio-economic development and increased water/food security in the SADC region. By understanding the resilience of groundwater resources, robust and informed strategies for water equality and GDP growth in the SADC region can be envisioned and implemented. |
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0022-1694 |
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THL @ christoph.kuells @ rooyen_using_2022 |
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94 |
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Author |
Xu, W.D.; Burns, M.J.; Cherqui, F.; Duchesne, S.; Pelletier, G.; Fletcher, T.D. |
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Title |
Real-time controlled rainwater harvesting systems can improve the performance of stormwater networks |
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Journal Article |
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2022 |
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Journal of Hydrology |
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614 |
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128503 |
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Real-time control, Rainwater harvesting systems, Stormwater control measures, Flood mitigation, Source Control, Climate change |
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Abstract |
Real-Time Control (RTC) technology is increasingly applied in Rainwater Harvesting (RWH) systems to optimise their performance related to water supply and flood mitigation. However, most studies to date have focussed on testing the benefits at an individual site scale, leaving the potential benefits for downstream stormwater networks largely untested. In this study, we developed a methodology to predict how at-source RTC RWH systems influence the behaviour of a stormwater network. Simulation was enabled by coupling the drainage model in SWMM with an RTC RWH model coded using the R software. We modelled two different RTC strategies across a range of system settings (e.g. storage size for RWH and proportion of storage to which RTC is applied) under two different climate scenarios—current and future climates. The simulations showed that RTC reduced flooding volume and peak flow of the stormwater network, leading to a potential mitigation of urban flooding risks, while also providing a decentralised supplementary water supply. Implementing RTC in more of RWH storages yielded greater benefits than simply increasing storage capacity, in both current and future climates. More importantly, the RTC systems are capable of more precisely managing the resultant flow regime in reducing the erosion and restoring the pre-development conditions in sensitive receiving waters. Our study suggests that RTC RWH storages distributed throughout a catchment can substantially improve the performance of existing drainage systems, potentially avoiding or deferring expensive network upgrades. Investments in real-time control technology would appear to be more promising than investments in detention volume alone. |
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0022-1694 |
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Call Number |
THL @ christoph.kuells @ Xu2022128503 |
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233 |
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